You might want to consider misusing the Xe-chamber which a couple of labs and 
synchrotrons bought in the late 90's to derivative crystals with Xenon. Instead 
of flushing the chamber with Xenon you could flush it with CO2 then plunge 
freeze your crystals within the chamber.

careful advertisement follows:
http://hamptonresearch.com/product_detail.aspx?cid=21&sid=121&pid=346
[/clicking on links provided through emails are at your own risk/]

Jürgen

On Oct 2, 2011, at 6:36 PM, Edward A. Berry wrote:

Jacob Keller wrote:
Dear Crystallographers,

I would like to soak my crystals in bicarbonate (a possible
substrate), but the crystals have grown--and only grow--in pH 5.2-6.0,
so the bicarb/CO2 will just keep evolving out of the solution and
reliquishing its hydroxyls until the pH is elevated sufficiently out
of range. Does anyone have a clever way of getting bicarb into these
crystals? Grow them under CO2? Transfer them to higher pH, and hope
for the best?

Jacob Keller

Assuming they grow by vapor diffusion- how about:
Replace the reservoir with diet coke (Perrier water
if you want to be high class) with pH adjusted to
the range you want and sufficient PEG or glycerol
to give the same osmolarity?
CO2 diffusing in will lower the pH but not much below
that of the reservoir. When you open the well to mount,
especially with hanging drops, the CO2 will leave
and pH will rise, but not above the starting point.

......................
Jürgen Bosch
Johns Hopkins University
Bloomberg School of Public Health
Department of Biochemistry & Molecular Biology
Johns Hopkins Malaria Research Institute
615 North Wolfe Street, W8708
Baltimore, MD 21205
Office: +1-410-614-4742
Lab:      +1-410-614-4894
Fax:      +1-410-955-2926
http://web.mac.com/bosch_lab/





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