Thought of this originally but the peak is almost on top of the Sulfur and with 
the oddly high B value I don’t think it is that.   I would also think it would 
show up on both monomers vs just one.

Len


On Aug 10, 2022, at 10:26 AM, Roger Rowlett 
<[email protected]<mailto:[email protected]>> wrote:

Do you mean the sulfur atom density is larger, or do you mean there is a 
density peak adjacent to the sulfur atom? It is possible for cysteine (CYS) 
residues to be oxidized to S-hydroxycysteine (CSO) under certain storage or 
crystallization conditions. Ran into this in a cysteine hydrolase structure.

Roger Rowlett
Gordon & Dorothy Kljne Professor, Emeritus
Department of Chemistry
Colgate University

On Wed, Aug 10, 2022, 11:00 AM Thomas, Leonard M. 
<[email protected]<mailto:[email protected]>> wrote:
Hello All,

I have run into something odd.  In working on a structure for one of the groups 
I work with regularly, on one of the cystine residues I have a very large 
positive density peak at the sulfur position. The B value is approximately 4 
times the other values in the residue and on other cystine residues.  The 
overall structure has 2 molecules in the asymmetric unit  and the corresponding 
cystine  on the other monomer is behaving as I would expect.   There are no 
disulfides in the structure.

The data were collected on 9-2 at SSRL and all three of the data sets we 
collected show the same thing, all data go to about 2.2 angstroms.  We are 
trying to determine the ligand binding in the molecule but this cystine is not 
involved in ligand binding.  In house and other synchrotron data from previous 
protein preps and data collection runs of the same molecule grown in very 
similar condition and crystallized in the same space group have the residue 
behaving normally.

I am open to any ideas as to what may be going on as I am rather puzzled by 
this.

Thanks for any input,
Len Thomas

Leonard Thomas, Ph.D.
Biomolecular Structure Core, Director
Oklahoma COBRE in Structural Biology
Price Family Foundation Institute of Structural Biology
University of Oklahoma
Department of Chemistry and Biochemistry
101 Stephenson Parkway
Norman, OK 73019-5251
Office: (405)325-1126
[email protected]<mailto:[email protected]>
http://www.ou.edu/structuralbiology/cobre-core-facilities/mcl


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