Response to the question regarding pH-induced colour shifts in organic dyes
on paper, posted by Fiona McLees in vol. 33 issue 28:

I was recently part of a research project focused on a photo album from the
Tropenmuseum in Amsterdam, whose coloured album pages display intense local
discolouration caused by contact with an alkaline adhesive. The album paper
is of a dark, olive-grey colour and the areas damaged by the adhesive
appear bright yellow-orange.

The colourants in the paper were identified as synthetic dyes of the
triarylmethane and azo classes. The damaging adhesive was identified as a
mixture of starch with sodium silicate, a highly alkaline compound also
known as waterglass.

Although the research could not fully explain the discolouration, it seems
like the high pH of the damaging adhesive mostly affected
the triarylmethane dyes, while the azo dyes underwent only minor changes.
Triarylmethane dyes are known to shift colour depending on pH conditions.
In aqueous media, these colour shifts are theoretically reversible, but
it's not clear what happens when these dyes are used on paper and how the
substrate affects the discolouration process.

It's great to hear of new studies looking into pH-induced colour changes on
paper! I would be happy to send more information on my research to anyone
interested in this topic.

Andra Danila
Paper Conservator in Training
University of Amsterdam
[email protected]
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