I’ve just been following the group for a couple of weeks now. A few
thoughts:

1. First, taking up on Mike’s previous discussion (Hi, Mike) of a
localized use of SRM for the arctic, I am wondering about the
following (perhaps you’ve already discussed this, apologies if so): a
possible complication seems to me that you could potentially get
improved surface temperature and ice cover as desired, but still have
rapid destabilization of shelf submarine methane hydrates continuing
on, relatively unabated, for quite some time, depending on its precise
dynamics. Maslowski’s modelling is generally driven by a lot of warm
water getting in at the Bering Strait, which seems logical enough, and
might explain the hydrate changes, but some imagine a geothermal
cause, and there’s lots of riverine inflow, too, and warmer water
coming in via Fram Strait/Barents Sea as well. It would seem important
to figure out what is happening with all that, and then, if Maslowski
were right, let’s say, it could help to extend the area of injection
down into the north pacific (or perhaps some other element to a ‘mixed
plan’ could be added to grapple with the problem). Anyhow, doesn’t it
seem possible that although the shelf is very shallow, changing what’s
happening at the surface alone might not be extremely effective for
this part of the problem (and a chief raison d’etre for urgent action
to begin with) if warm water is directly spilling into the shelf area
through lower currents that remain unchanged. Or am I wrong, and is
this not a significant concern?

2. On a ‘soft’ geoengineering note, I organized some testing at UVA on
TiO2 activity on methane. We have found that it is possible to
photocatalytically activate methane in ambient conditions with TiO2,
but it is quite a weak reaction, and we do not think it is really
usable as it is. I’m now looking at a possible co-catalyst (Mo is my
prime interest). The lab at UVA (Lehmann lab) has great precision in
reading methane (to ppt level), but not a lot of expertise with
something like calcination of new catalysts, etc. If anyone knows of
some lab that might like to help – we would provide detailed
experimentals (from an early Graetzel paper), which would be easy
stuff for many labs.  Of course, TiO2 ‘environmental coatings’ work
very well on VOCs, NOx, etc., as they are – but since those have
opposing signs, it seems to me that it would have little net effect on
RF, even if healthy for the air. The idea would be to get something
with -RF that could be added to the surface of the white roof
projects, etc. The TiO2 coatings have self-cleansing properties, and
so should help boost the reflective surface as well, and on those
grounds alone the idea of adding such coatings is already spreading.
Perhaps altering the TiO2 catalyst so it is just more selective for
NMVOC (but not NOx) would be an alternate route? It wouldn’t save the
world, but it could be something practical that would be very likely
(I’d guess close to 100%, since such coatings are probably going to be
added in any case) to actually get done soon if it could be developed.
Any thoughts?

3. In the opposite direction, looking at much more highly invasive
measures, here’s a different idea, which I haven’t heard before, and
which I only mention with that sense that a ‘think tank’ is all about
a willingness to say stupid things! So, forgive me:  I remember once
talking to a researcher who works on arctic halogen chemistry, who
mentioned to me that the reaction of atomic chlorine with methane is
some 60x greater than hydroxyl’s. While I know that this might seem
like a rather ‘insensitive,’ imagine in the equatorial tropopause,
where methane is prevalent and thus somewhat longer lived, some kind
of aircraft (or perhaps balloon-based) spraying of ∙Cl over the marine
environment. The very strong reaction, Cl+CH4→ClH+CH3 means that
hydrochloric acid would be the chief polluting product (the methyl
radical would have gotten made eventually in methane hydroxylation),
which is apparently a not insignificant part of sea-salt induced rain
anyhow (a total deposition of 1.8-5 Tg/yr of nssHCl is estimated, I’ve
read). I’m sure there would likely be plenty of other unwanted
products, though. Some would surely get up to the stratosphere, but
the ozone layer is less affected there, and that at least still has a
negative forcing. One might say that if you took a low multiple of
natural HCl level as a tolerated pollution limit – say a doubling or
tripling of natural levels – then the amount of methane that could be
reacted in making that much HCl might be considered ‘safe.’Any
thoughts?

4. I know many people have at times suggested various marine floating
things – I remember David Keith mentioning somewhere that oceanic
reflective particles were in the very first U.S. government-
commissioned study mentioning geoengineering, some 40 years ago. But
for helping arctic ice, has there been research yet on things like the
following? EPS and polyethylene are so abundant in landfills, and so
buoyant. Imagine something with four legs (made of EPS coated in
polyethylene), and then a polyethylene body staying a couple feet
above the water surface, say 12 ft sq., or as large as could be
structurally sound, with a reflective (white EPS) surface. It could
have some kind of intermittent siding as wind-breaker. Thus it would
allow heat dissipation, provide shade for the surface, reflect
sunlight, and break the wind. It would not pollute the water much,
since the body would be suspended. While it would be quite motile,
might it not, where situations were near criticality, help ice
creation/survival? Maybe placed in the southern Beaufort Sea, or just
north of the Bering Strait, such a thing could prove strategically
helpful?


Yesterday, Ken’s response 'C.' on the ETC Group report got Josh to say
that the “either/or” problems of moral hazard in geoengineering should
be solved by the “wedge” concept, both in the sense of including
geoengineering in the mix (of course, white roofing, hopcalite
catalysts on car radiators, etc, mean it already is, albeit quietly)
and within the geoengineering domain itself – i.e., a wide portfolio
of different modest-sized possible geoengineering projects would be
best. I strongly support that viewpoint. I would think that a goal for
modeling would be to design a program to show at any time what the
currently agreed to patchwork of emissions reductions will provide,
how many Wm-2 we will likely need by when in excess of that, and then
be able to show different options for getting there through a variety
of pathways.

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