Unless I have misunderstood it, the website requires a password to view these 
papers and the email given to request a password has not responded in a week or 
so . Could you give me/us  a password.

I am of course very interested in alternatives to SO2 as a way of producing 
aerosols because of my proposal for tetra ethyl silicate in aircraft fuel to 
produce silica particles. Even if the fuel cant be burnt in the jet engine and 
needs a special burner, the storage and pumping would just use the existing 
equipment. Laboratory research project proposal at 
http://www.naturaljointmobility.info/grantproposal09.htm 

Having looked at the various proposals for producing stratospheric aerosols, I 
think mine might well be the quickest to get into experimental operation. 
(Obviously we should get all viable proposals ready for experimental 
atmospheric implementation) If anyone can get some money for lab experiments I 
will cooperat fully.

john gorman

  ----- Original Message ----- 
  From: David Keith 
  To: [email protected] ; [email protected] 
  Sent: Thursday, September 02, 2010 10:06 PM
  Subject: [clim] Several papers


  This is a shameless advert for new papers on the science and policy of solar 
radiation management.  

   

  The papers are available from the preprint section of my website 
(www.ucalgary.ca/~keith/Preprints.html, earlier geoengineering papers and talks 
are at www.ucalgary.ca/~keith/geo.html) 

   

  Two papers are publishing in the next couple of weeks (The PNAS paper 
publishes Tuesday, it is embargoed until then, and the GRL paper is already on 
their website in preprint form, but it will be a few weeks before formal 
publication.)

   

  Jeffrey R. Pierce, Debra K. Weisenstein, Patricia Heckendorn, Thomas Peter 
and David W. Keith. Efficient formation of stratospheric aerosol for climate 
engineering by emission of condensable vapor from aircraft. Geophysical 
Research Letters. 

  Copying volcanoes by injecting SO2 doesn't work very well because most of the 
added sulfur is deposited on the largest particles, producing the particle size 
distribution that is too large. Direct injection of sulfuric acid from an 
aircraft can allow much better control of particle size distribution. In our 
un-optimized models, it looks like this method can reduce the amount of sulfur 
needed to achieve 4 Wm-2 by more than a factor of two, and by a much larger 
factor when compared with injection of SO2 near the equator. Similar methods 
might be employed for other condensable vapors using technologies had been well 
explored in vapor phase fabrication of nano-scale particles. 

  Note that: A preliminary look at the engineering suggest that these methods 
do not require any technological leap. Note also, that we have commissioned a 
study of delivery methods by aircraft engineering company and will release the 
entire report in the next month or so.

   

  David W. Keith. Photophoretic levitation of engineered aerosols for 
geoengineering. Proceedings of the National Academy of Sciences.

  Engineered nanoparticles could exploit photophoretic forces, enabling more 
control over particle distribution and lifetime than is possible with sulfates, 
perhaps allowing climate engineering to be accomplished with fewer side 
effects. The use of electrostatic or magnetic materials enables a class of 
photophoretic forces not found in nature. Photophoretic levitation could loft 
particles above the stratosphere, reducing their capacity to interfere with 
ozone chemistry; and, by increasing particle lifetimes, it would reduce the 
need for continual replenishment of the aerosol. Oriented particles can be 
non-spherical allowing backscatter with essentially none of the forward 
scattering caused by small spherical aerosols.  Moreover, particles might be 
engineered to drift poleward enabling albedo modification to be tailored to 
counter polar warming while minimizing the impact on equatorial climates. 

   

  Note: While cost and feasibility of producing and dispersing of such 
particles is unknown, analogies to existing particle fabrication technologies 
suggest that such methods cannot be dismissed out of hand. More generally, this 
suggest that there might be a range of technically sophisticated options beyond 
mimicking volcanoes that might offer advantages in the form of more 
controllable climate forcing, the downside is that it's far easier to think of 
new methods than it is to understand their effectiveness of environmental risks.

   

  The following two papers are under review at Climatic Change, but since their 
review process is long I want to make them available as preprints:

   

  Juan Moreno-Cruz, Katharine Ricke and David W. Keith, A simple model to 
account for regional inequalities in the effectiveness of solar radiation 
management. Submitted to Climatic Change.

  We calculate the amount of SRM that minimizes impacts using three different 
social objectives: egalitarian, utilitarian and ecocentric.  While inequalities 
in the effectiveness of SRM between regions are important, they may not be as 
severe as is often assumed.  When changes in precipitation and temperature are 
normalized by pre-industrial variability and weighted equally, we find that SRM 
could compensate for most of the damages caused by carbon-dioxide-driven 
climate change without making any region worse-off. While this method provides 
a parsimonious way to examine inequality, quantitative conclusions will require 
more realistic estimates of impact and of the climate's response to SRM. 

  Put simply: This method helps describe inequalities, but we need to look at 
the effectiveness of SRM on actual impacts such as crop productivity, sea level 
rise, availability of surface water etc, rather than the stuff that's 
convenient for climate modelers such as annual average temperature and 
precipitation treated independently. 

   

  Juan B Moreno-Cruz and David W Keith. Climate Policy under Uncertainty: A 
Case for Geoengineering. Climatic Change.

  We introduce SRM in a model of climate change economics and analyze the 
optimal policy under uncertainty. We find that the quick response allowed by 
SRM makes it important even if it is relatively ineffective at compensating for 
CO2-driven climate change or even if its costs are expected to be large 
compared to traditional mitigation strategies. Finally, we examine the 
implications of uncertainty about the effectiveness of SRM and show that the 
value of reducing this uncertainty can readily exceed several trillion US 
dollars over the next 100 years, providing a strong argument for a research 
program.

   

   

  David Keith
  Canada Research Chair in Energy and the Environment 

  www.ucalgary.ca/~keith
  [email protected]
  (403) 220-6154

   


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