Thanks for the responses - though what I had in mind was actually more
in line with the tenor of Mike's latest comments about the 6-to-1
lifetime ratio for arctic sulfur SRM, stratospheric vs. tropospheric,
etc.

David’s early article is very impressive for how much it adumbrated
the current public discourse on geoengineering, though at the same
time, a bit of misunderstanding about what I was intending to ask –
and I was probably not expressing myself very well – possibly
underscores how something really has been shifting lately within the
geoengineering world, too. What I meant about tropospheric sulfur
injections was entirely in the newer sense of a more ‘localized
geoengineering’, which has been getting attention here in this group
lately (so much so that I forgot to mention what I meant in my
question), and which I think makes a world of difference in
considering its use. In a sense, stratospheric injections can’t be
effectively localized, and this newer local thinking - coming in
response to events on the ground - might bring out new ways of
considering tropospheric sulfur versus stratospheric sulfur, as Mike’s
comments from earlier today in that other thread show, and the issue
of sulfur's dangers, which are the main point in David's comments, are
clearly altered by the reduced scale of use.

In the BBC article that Andrew has just posted, Pete Wadhams is
talking about AMEG’s plans should the methane situation there
deteriorate a good deal further (which seems almost certain, if I had
to guess), and they focus on MCB alone. I think I had first seen
mention here of tropospheric sulfur injections in this context from
Mike, and this really took off in my imagination when I by chance
shortly afterward saw some work involving Eileen Matthews (Gauci et
al) showing how strongly just ordinary levels of acid rain will impede
methanogenesis in wetlands, with strong reductions, like 40% or so,
which play out through considerably longer time periods than the brief
atmospheric lifetime of the aerosols.

I think study of this combined methane-SRM effect for tropospheric
sulfur injection should really be done. Curiously, David, in what you
sent me, the abstract on intercontinental effects of SO2 don’t suggest
that Russia is particularly bad for that particular concern, less so
than Europe, for example. And curiously, I might add, despite what you
just wrote, in your early paper you had actually listed stratospheric
injections as more dangerous than tropospheric (although I assume for
entirely different reasons, related then to ozone loss concerns, etc).

But this is really something very different now from all that, or from
Budyko’s early comparisons of efficiency, lifetimes, etc. We’re
talking about a very limited area for treatment, almost nothing by
comparison with plans to geoengineer a global –1W/m2 or some such
thing. And currently one third of the land area of China is
experiencing acid rain, I recently read. How could it be acceptable to
add copious amounts of sulfur to one of the most densely populated
parts of the planet, which will clearly lead to considerable mortality
and sickness, and unacceptable to add any sulfur at all to a mostly
unpopulated area around the mouth of the Lena river, where there are
globally dangerous submarine methane hotspots and lots of wetlands,
thermokarst lakes, etc, emitting plenty of methane right nearby?

Could one not hope that there might be some effect from the sulfur on
the shelf floor itself, too? (I've cc-ed Vincent Gauci on this, and
maybe he could easily answer that).  After all, it is a complex
picture at the ESAS, probably with older methane stores and current
methanogenesis from thawing submarine permafrost driving the ambient
methane levels' rise there together. Indeed, the isotopic analysis
thus far points more to contemporary methane, which might
realistically be capable of being impacted – so it might be possible
to help push back against this spiraling situation in multiple
respects at once simply through tropospheric emissions of sulfur. That
is, with pinpointed and targeted ground level injections, there’s the
scattering effect – less efficient than in the stratosphere but still
certainly present – then the indirect effect (its ‘Twomey’ effect),
and then its methane-suppressing effects as well. Someone should try
to roughly calculate what might be possible totals in terms of local –
RF, given different options for release area, amount of release per
hour, estimates of what the wetlands near the hotspots are currently
emitting, etc.

Further, since it sounds from the BBC article as though MCB is the
main thing being considered by AMEG right now, another question of
mine would be for John, and that is how would the interaction of such
ground-level sulfur injection and the MCB compare to the rather
synergistic situation of MCB with stratospheric injections? (I noticed
that Wadhams is proposing MCB down around the Diomedes, though). I
realize that’s probably got to be a complex answer.

In terms of the sulfur’s dangers, like Paracelsus’ old saying, “The
poison is the dose.” The US still emits about 2/3rds of the SO2 it did
back in 1980, but mortality here has, I believe, been lowered a great
deal more than a third (I couldn't find current numbers for US deaths
from sulfur pollution, though). Obviously, as David himself pointed
out, since it would be done explicitly for its RF effect, too, there
would be a good deal of capacity to control its releases to prevent
harm from taking place as much as possible (although there are always
going to be temporary negative ecological impacts, I realize, too).

I would gather it would also be much easier to bring such a plan to
deployment, in terms of governance issues, public acceptance, etc,
than anything done involving the stratosphere.

All Best, Nathan



On Mar 17, 8:43 am, Veli Albert Kallio <[email protected]>
wrote:
> The size of the termination shock is likely to be comparable to the graph 
> when temperatures were suppressed from 1940-1970 when sulphur emissions were 
> rising. The acid rains were starting to destroy forests (the Black Forest in 
> Germany) and the acidity of Sweden's and Finland's lakes were rising rapidly. 
> UK had western winds that pushed most of sulphur into Sweden and some of it 
> to the Baltic countries and Finland. Nickel and Murmansk industries in the 
> Arctic caused widespread dead zones in the Kola Peninsula, in Russia that 
> lies north-east of Finland. The quantity increases of sulphur may have 
> occurred, but it would push the warming 30 years ahead of schedule if we 
> follow figures from 1940-1970. Events that could lead to a sudden switch off 
> of energy system using sulphur fuels could be a nuclear war or event like 
> sudden Greenland ice sheet land containment failure leading to Heindrich Ice 
> Berg Calving Event and the North Atlantic Ocean to be filled by broken ice 
> bergs and the onset of the Last Dryas. However, both nuclear winter and the 
> Last Dryas would mitigate the warming effect by strong negative feedbacks in 
> either scenario. A sudden sea level jump by few metres would also tear off 
> ice shelves by bending them loose around Antarctica. This replicates the 
> cooling of Northern Hemisphere to the Southern Hemisphere. Droughts would be 
> unbearable in both cases as the oceans would be very cold while the global 
> dimming effect would be lost over the continent. The Atlantic regions would 
> be affected by cold and drought, and much of eastern parts of Eurasia would 
> suffer loss of monsoon and very low precipitation. Large ice bergs resulted 
> in above kind of event are so-called ice islands and these can take 15 years 
> to melt away. During this period the ocean remains perennially cold and may 
> be Finland could re-introduce its reindeer and musk ox stocks across the 
> mainland Europe to supply meat. As a positive point the Central Europe could 
> enjoy a period of beautiful Arctic flowers such as Dryases that like the cold 
> weather and decorate our Arctic summer each year. Regards, Albert
>  Date: Sat, 17 Mar 2012 09:59:10 +0000
> Subject: RE: [geo] tropospheric aerosol use
> From: [email protected]
> To: [email protected]
> CC: [email protected]; [email protected]; [email protected]
>
> Another point to note is that tropospheric sulfur geoengineering is already 
> being done, albeit inadvertently, by power plants, ships and factories.
> If we stop this, we will have a termination shock, as was reported 
> numerically on this list recently wrt the US (possibly by Kens group).
> A further termination shock will arise from secondary effects on marine 
> clouds. This was reported at IUGG, but observationally rather than 
> numerically. I've not seen the paper.
> We are therefore just about to commence a poorly researched geoengineering 
> programme to heat up the planet a bit!
> A
> On Mar 17, 2012 3:53 AM, "John Latham" <[email protected]> wrote:
>
> Hello All,
>
> Budyko’s points – re tropospheric vvs stratospheric aerosol -  reiterated
>
> by Govindasamy Bala (below), in response to Nathan Currier’s question
>
> (also below) are clearly valid vis-à-vis cooling via scattering of solar
>
> radiation and concomitant global cooling.
>
> However, it does not follow that the effectiveness of stratospheric seeding is
>
> greater than that of the Marine Cloud Brightening (MCB) geo-eng technique,
>
> which involves the (tropospheric) seeding of marine stratocumulus clouds
>
> with sea-water aerosol, in order to increase their droplet number
>
> concentration, and therefore their albedo (with concomitant global cooling).
>
> Latham et al (2008) presented arguments indicating that the ratio of the rate 
> of
>
> planetary radiative loss to required operational power is very large (in the
>
> range 10**5 to 10**7 according to the type of vessel used for the continuous
>
> spraying required). They pointed out that the main reason why this ratio is so
>
> high for MCB is that Nature provides the energy required for the increase of
>
> surface area of newly activated cloud droplets by 4 or 5 orders of magnitude
>
> as they ascend to cloud top and reflect sunlight.
>
> All Best,    John.
>
> John Latham
>
> Address: P.O. Box 3000,MMM,NCAR,Boulder,CO 80307-3000
>
> Email: [email protected]  or [email protected]
>
> Tel: (US-Work) 303-497-8182 or (US-Home) 303-444-2429
>
>  or   (US-Cell)   303-882-0724  or (UK) 01928-730-002
>
> http://www.mmm.ucar.edu/people/latham
>
> ________________________________________
>
> From: [email protected] [[email protected]] on 
> behalf of Govindasamy Bala [[email protected]]
>
> Sent: Friday, March 16, 2012 3:52 AM
>
> To: [email protected]
>
> Cc: geoengineering
>
> Subject: Re: [geo] tropospheric aerosol use
>
> "Climate changes" by Budyko, on page 244, discusses why tropospheric aerosols 
> are not as effective as stratospheric aerosols for climate modification.
>
> 1) life time is only a couple of weeks
>
> 2) Particle size becomes too big quickly and hence not effective for 
> scattering
>
> 3) Presence of clouds make them less effective
>
> 4) absorption by aerosols of near IR shortwave could partially cancel the 
> cooling by scattering.
>
> Bala
>
> On Thu, Mar 15, 2012 at 9:53 PM, Nathan Currier 
> <[email protected]<mailto:[email protected]>> wrote:
>
> Does anyone know of any published papers exploring the use of
>
> tropospheric aerosol use?
>
> cheers,
>
> Nathan
>
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> Best wishes,
>
> -------------------------------------------------------------------
>
> Dr. G. Bala
>
> Associate Professor
>
> Center for Atmospheric and Oceanic Sciences
>
> Indian Institute of Science
>
> Bangalore - 560 012
>
> India
>
> Tel: +91 80 2293 3428
>
>         +91 80 2293 2075
>
> Fax: +91 80 2360 0865
>
>         +91 80 2293 3425
>
> Email: [email protected]<mailto:[email protected]>
>
>              bala.gov<http://bala.gov>@gmail.com<http://gmail.com>
>
> Web:http://caos.iisc.ernet.in/faculty/gbala/gbala.html
>
> -------------------------------------------------------------------
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