Atmos. Chem. Phys., 12, 3349-3362, 2012
www.atmos-chem-phys.net/12/3349/2012/
doi:10.5194/acp-12-3349-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.

Climatic effects of 1950–2050 changes in US anthropogenic aerosols – Part 2: 
Climate response

E. M. Leibensperger1,*, L. J. Mickley1, D. J. Jacob1, W.-T. Chen2, J. H. 
Seinfeld3, A. Nenes4, P. J. Adams5, D. G. Streets6, N. Kumar7, and D. Rind8
1School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, 
USA
2Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, 
USA
3Division of Chemistry and Chemical Engineering, California Institute of 
Technology, Pasadena, CA, USA
4School of Earth & Atmospheric Sciences and School of Chemical & Biological 
Engineering, Georgia Institute of Technology, Atlanta, GA, USA
5Department of Civil & Environmental Engineering and Department of Engineering 
& Public Policy, Carnegie Mellon University, Pittsburgh, PA, USA
6Argonne National Laboratory, Argonne, IL, USA
7Electric Power Research Institute, Palo Alto, CA, USA
8NASA Goddard Institute for Space Studies, New York, NY, USA
*now at: Dept. of Earth, Atmospheric and Planetary Sciences, Massachusetts 
Institute of Technology, Cambridge, MA, USA

Abstract. We investigate the climate response to changing US anthropogenic 
aerosol sources over the 1950–2050 period by using the NASA GISS general 
circulation model (GCM) and comparing to observed US temperature trends. 
Time-dependent aerosol distributions are generated from the GEOS-Chem chemical 
transport model applied to historical emission inventories and future 
projections. Radiative forcing from US anthropogenic aerosols peaked in 
1970–1990 and has strongly declined since due to air quality regulations. We 
find that the regional radiative forcing from US anthropogenic aerosols elicits 
a strong regional climate response, cooling the central and eastern US by 
0.5–1.0 °C on average during 1970–1990, with the strongest effects on maximum 
daytime temperatures in summer and autumn. Aerosol cooling reflects comparable 
contributions from direct and indirect (cloud-mediated) radiative effects. 
Absorbing aerosol (mainly black carbon) has negligible warming effect. Aerosol 
cooling reduces surface evaporation and thus decreases precipitation along the 
US east coast, but also increases the southerly flow of moisture from the Gulf 
of Mexico resulting in increased cloud cover and precipitation in the central 
US. Observations over the eastern US show a lack of warming in 1960–1980 
followed by very rapid warming since, which we reproduce in the GCM and 
attribute to trends in US anthropogenic aerosol sources. Present US aerosol 
concentrations are sufficiently low that future air quality improvements are 
projected to cause little further warming in the US (0.1 °C over 2010–2050). We 
find that most of the warming from aerosol source controls in the US has 
already been realized over the 1980–2010 period.

Final Revised 
Paper<http://www.atmos-chem-phys.net/12/3349/2012/acp-12-3349-2012.pdf> (PDF, 
1342 KB)   Discussion 
Paper<http://www.atmos-chem-phys-discuss.net/11/24127/2011/acpd-11-24127-2011.html>
 (ACPD)

Citation: Leibensperger, E. M., Mickley, L. J., Jacob, D. J., Chen, W.-T., 
Seinfeld, J. H., Nenes, A., Adams, P. J., Streets, D. G., Kumar, N., and Rind, 
D.: Climatic effects of 1950–2050 changes in US anthropogenic aerosols – Part 
2: Climate response, Atmos. Chem. Phys., 12, 3349-3362, 
doi:10.5194/acp-12-3349-2012, 2012.

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