But doesn't the question whether CaCO3 formation is a net source or sink of 
atmospheric CO2 depend on where the bicarbonate comes from? 

If CO2(aq, recently from atm) + H20 --> H2CO3  --> HCO3- + H+  is the source of 
the HCO3-, as at present in the Southern Ocean, then there is a net sink of one 
carbon. As the equation below requires two bicarbonate ions, 2C from atmosphere 
& 1C returns to atmosphere, there is a net sink of one carbon. 

It seems a blanket statement that CaCO3 formation emits CO2 presumes an 
infinite oceanic capacity to hold bicarbonate. Is that true? Doesn't increasing 
bicarbonate eventually degrade the ocean's H+ buffering function?

Some may consider ocean acidification to be a more existential threat than 
greenhouse warming, in the unknown unknown category.


----- Original Message ----- 
  From: Ken Caldeira 
  To: [email protected] 
  Cc: [email protected] ; [email protected] 
  Sent: Saturday, January 05, 2013 1:49 PM
  Subject: Re: [geo] Geoengineering: rules needed for climate-altering science 
- International institute for Strategic Studies


  Russell has his facts right but chemical implications wrong:


  The net reaction for the formation of CaCO3 shells can be written:


  Ca2+ + 2 HCO3-  ===>  CaCO3 + H2O + CO2


  Thus the formation of carbonate minerals from sea water acts as a carbon 
source to the atmosphere, not a sink.


  Greg Rau, among others, has proposed trying to run this reaction to the left 
to sequester CO2. This is sometimes known as "Accelerated Carbonate Weathering".


  http://crustal.usgs.gov/projects/CO2_sequestration/limestone.html




  _______________
  Ken Caldeira

  Carnegie Institution for Science 
  Dept of Global Ecology

  260 Panama Street, Stanford, CA 94305 USA

  +1 650 704 7212 [email protected]
  http://dge.stanford.edu/labs/caldeiralab  @kencaldeira


  Caldeira Lab is hiring postdoctoral researchers.
  http://dge.stanford.edu/labs/caldeiralab/Caldeira_employment.html

  Our YouTube videos
  The Great Climate Experiment: How far can we push the planet?  
  Special AGU lecture: Ocean Aciditication: Adaptive Challenge or Extinction 
Threat?
  More videos



  On Sat, Jan 5, 2013 at 10:12 AM, Russell Seitz <[email protected]> wrote:

    Given the proximity of  so many of ISIS proncipal to Chesapeake Bay, I am 
shocked they have not hit on the opportunity to combine the Beltway's lust to 
regulate with the best features of carbon capture and SRM.  


    The key to this win-win-win strategem is the humble mollusc Ostrea edulis.


    A dozen oysters sequester a hundred grams or more of carbon in their 
shells, and were the daily consumption of a dozen made mandatory, their removal 
from the sea would make room for the sequestration of a hundred grams more. In 
addition, discarding the shells on land  would at once take a bite out of sea 
level rise, and, as ouster shells are pearly white , tend to reduce the albedo 
footprint of those consuming them, especially if they toss them on their 
asphalt coated roofs, parking lots and driveways to reduce the energy toll  and 
radiative forcing burden of the urban heat island effect .


    Confident that perfoming the dimensional analysis necessary to persuade 
themselves of the relative worth of this concept will encourage readers to do 
likewise to their own submissions   I remain 



    Your , etc. 





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