David

Below are a few questions and comments from your interesting lecture today.
I'm copying to the Google group to invite wider comment on the important
issues your raised.

It would be great to hear any comments you have, if you are able to
respond.

Thanks

A

Ramp up
You considered a linear and shallow ramp up of SRM intervention. This
perhaps works particularly well for a linear climate response. Should we
not instead be looking at more rapid temperature reductions, to reduce
risks of crossing tipping points (Greenland, permafrost, etc)?

Health impacts
You assume quantifiable health impacts from particulate rain out. However,
the aerosol rain out would be well distributed, with much occurring in
depopulated areas. Are the health impacts of distributed particulates
comparable to those from concentrated loading patterns (eg focussed on
harbours and cities)?  I assume the calculated risks were derived from
these concentrated loading patterns. Will the health risks  be reduced
because rain out will likely mix with, or condensate, raindrops -  hence
diluting them to destruction.

Delivery mechanism
Previously you considered homogeneous condensation of H2SO4, and today you
discussed in-situ high-altitude combustion of solid S to release SO2. In
response to my verbal question, you stated that particle size distribution
issues only kick in around 'a few' MT. However, having a constant delivery
mechanism reduces the risk of 'nasty surprises' on switching, despite
increased lofting costs in earlier stages. Is there an argument for
'starting as you mean to carry on'?

Distribution pattern
Particularly with high aerosol loads, there may be advantages to a
temporally bound injection regime (when using precursor gases instead of
direct particulate injection). This is due to the benefit of constrained
particle growth. (See reference below) Does a potential requirement for a
temporally-concentrated injection regime mean that the use of aircraft
becomes problematic from a cost point of view? EG to do all the injection
in a month per year, you'd likely need up to 12x as many aircraft.
You also considered the spatial distribution pattern. A 30N to 30S
injection regime may take advantage of the Brewer Dobson circulation.
However, is there not a risk of particle size growth and rain out. See
Heckendorn et al ( http://m.iopscience.iop.org/1748-9326/4/4/045108 ), who
discussed particle growth, and I recall this paper may also have discussed
spatial (vertical and latitude) and temporal distribution patterns, and
advocated a more spatially varied injection regime.

Smart particles
You touched on the concept of 'smart particles'. Is there a risk that these
can be weaponised to make a solar concentrator, capable of burning
buildings on the ground?

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