http://dcgeoconsortium.org/2014/03/24/wil-burns-carbon-dioxide-removal-approaches-long-term-implications-and-requisite-societal-commitments/

(apologies for lost formatting. Best read online)

wil burns- carbon dioxide removal approaches: long-term implications and
requisite societal commitments

In recent years, a number of climate changecommentators, non-governmental
organizations, and intergovernmental organizations have discussed the
potential need for so-called "negative greenhouse gas emissions"
strategies. It is also anticipated that Working Group III of the
Intergovernmental Panel on Climate Change will include a discussion of this
approach in its upcoming report pursuant to its contribution to the Fifth
Assessment Report. The rationale advanced for focusing on negative
emissions approaches are usually the threat posed by burgeoning emissions,
which could result in exceeding of critical climatic thresholds in a few
decades, as well as system inertia, which could lock in temperature
increases associated with radiative forcing for many centuries. The
processes that could effectuate permanent removal carbon dioxide from
Earth's atmosphere include air capture, bioenergy and carbon capture and
storage, ocean iron fertilization and soil mineralization, and are usually
classified as carbon dioxide removal (CDR) geoengineering approaches.In my
next few postings on the site, I'd like to highlight some of the excellent
peer-reviewed literature on carbon dioxide removal strategies that has been
released in the past few years. In 2010, Stanford professors Long Cao and
Ken Caldeira published a study in the journalEnvironmental Research
Letters (open access) that sought to assess both the long-term consequences
and level of commitment required to effectuate massive removal of carbon
dioxide from the atmosphere. The researchers employed a coupled-climate
carbon cycle model, initially integrated under a fixed pre-industrial
atmospheric concentration of 278ppm for 5000 years. The model was
subsequently integrated under prescribed historical carbon dioxide
concentrations between 1800-2008, and then forced with carbon dioxide
emissions from 2009-2049 following the IPCC's A2 emissions scenario. The
study then simulated cessation of carbon dioxide emissions and two extreme
carbon dioxide scenarios, one in which carbon dioxide was instantaneously
set to its pre-industrial level of 278ppm at the beginning of 2050 by
removing all carbon dioxide from atmosphere, with carbon dioxide levels in
the atmosphere permitted to evolve freely thereafter, and the other
scenario in which carbon dioxide was set at 278ppm in 2050 and then held at
that level thereafter. In both scenarios, integration of the simulations
was continued until 2500.Among the study's conclusions:Following an extreme
one-time removal of all anthropogenic carbon dioxide from the atmosphere,
atmospheric concentrations are restored under the simulation to
pre-industrial levels of 278ppm.However, due to efflux of carbon from land
associated with responses of net primary production and soil respiration,
as well as releases of carbon from oceans, atmospheric concentrations
experience an overshoot, with a peak concentration of 362ppm 30 years after
the removal.  Overall, 27% of removed carbon returns to the atmosphere.
Thus, if society would wish to maintain atmospheric concentrations of
carbon dioxide at a specified level, it would have to commit itself to
long-term removal of carbon dioxide released from land and ocean sources;A
one-time removal of anthropogenic carbon dioxide also reduces warming by a
little less than 50% at the time of removal, and radiative forcing by
two-thirds on centennial timescales.If atmospheric concentrations of carbon
dioxide were restored to 350ppm, it would result in surface warming of
1.2°C, which would last for several centuries;The simulated reduction in
temperatures in the study yields a cooling of 0.16°C for every 100 PgC CO2
removal. The conclusion that the concept of proportional temperature change
to cumulative carbon dioxide emissions is apposite to carbon dioxide
removal has implications for assessing the potential effectiveness of such
approaches.The study also contains a cautionary note: if effective heat
capacity should prove to be less than estimated in the study, or the carbon
dioxide degassing timescale proved longer, it could result in temperature
overshoots in which initial temperature decreases are reversed when carbon
dioxide re-accumulates in the atmosphere. However, the research concluded
that they did not observe this result in their simulations.Of course, it is
not likely that deployment of negative emissions approaches would, or in
the case of most prospective technologies, could, follow what the
researchers themselves characterize as an "extreme" scenario, i.e. a
one-time removal of all carbon dioxide at a discrete point. Moreover, it's
far from clear that society would seek to return to pre-industrial climatic
conditions, even if that could be effectuated. And, of course, the study
did not address issues associated with feasibility, However, this study is
very valuable for a number of reasons. First, it provides a preliminary
estimate of anticipated reductions in temperatures per 100 PgC CO2,
providing a guide to policymakers who might contemplate more limited uses
of negative emissions strategies than contemplated in this study. Second,
the study provides a pointed reminder of the fact that a negative emissions
strategy would likely necessitate a multi-generational societal commitment,
with all of the implications that this would hold for governance, ethics
and practical logistics. Finally, the study could provide students with an
excellent window into the methods, as well as challenges, of simulating the
climatic impacts of geoengineering strategies with climate models

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