http://rsta.royalsocietypublishing.org/content/372/2031/20140051

Modelling artificial sea salt emission in large eddy simulations

Z. Maalick, H. Korhonen, H. Kokkola, T. Kühn, S. Romakkaniemi
DOI: 10.1098/rsta.2014.0051
Published 17 November 2014

Abstract

We study the dispersion of sea salt particles from artificially injected
sea spray at a cloud-resolving scale. Understanding of how different
aerosol processes affect particle dispersion is crucial when designing
emission sources for marine cloud brightening. Compared with previous
studies, we include for the first time an explicit treatment of aerosol
water, which takes into account condensation, evaporation and their effect
on ambient temperature. This enables us to capture the negative buoyancy
caused by water evaporation from aerosols. Additionally, we use a higher
model resolution to capture aerosol loss through coagulation near the
source point. We find that, with a seawater flux of 15 kg s−1, the cooling
due to evaporation can be as much as 1.4 K, causing a delay in particle
dispersion of 10–20 min. This delay enhances particle scavenging by a
factor of 1.14 compared with simulations without aerosol water. We further
show that both cooling and particle dispersion depend on the model
resolution, with a maximum particle scavenging efficiency of 20% within 5 h
after emission at maximum resolution of 50 m. Based on these results, we
suggest further regional high-resolution studies which model several
injection periods over several weeks.

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