Poster's note : as far as I can tell, this is the revised version. This
research may be important in eroding the arguments for switching to other
aerosols

http://www.atmos-chem-phys.net/16/2843/2016/

Climatic impacts of stratospheric geoengineering with sulfate, black carbon
and titania injection

Anthony C. Jones, James M. Haywood, and Andy Jones

Received: 12 Oct 2015 –Published in Atmos. Chem. Phys. Discuss.: 03 Nov 2015
Revised: 25 Feb 2016 – Accepted: 26 Feb 2016 –Published: 04 Mar 2016

Abstract. In this paper, we examine the potential climatic effects of
geoengineering by sulfate, black carbon and titania injection against a
baseline RCP8.5 scenario. We use the HadGEM2-CCS model to simulate
scenarios in which the top-of-the-atmosphere radiative imbalance due to
rising greenhouse gas concentrations is offset by sufficient aerosol
injection throughout the 2020–2100 period. We find that the global-mean
temperature is effectively maintained at historical levels for the entirety
of the period for all three aerosol-injection scenarios, though there is a
wide range of side-effects which are discussed in detail. The most
prominent conclusion is that although the BC injection rate necessary to
produce an equivalent global mean temperature response is much lower, the
severity of stratospheric temperature changes (> +70 °C) and precipitation
impacts effectively exclude BC from being a viable option for
geoengineering. Additionally, while it has been suggested that titania
would be an effective particle because of its high scattering efficiency,
it also efficiently absorbs solar ultraviolet radiation producing a
significant stratospheric warming (> +20 °C). As injection rates and
climatic impacts for titania are close to those for sulfate, there appears
to be little benefit in terms of climatic influence of using titania when
compared to the injection of sulfur dioxide, which has the added benefit of
being well-modeled through extensive research that has been carried out on
naturally occurring explosive volcanic eruptions.

Citation: Jones, A. C., Haywood, J. M., and Jones, A.: Climatic impacts of
stratospheric geoengineering with sulfate, black carbon and titania
injection, Atmos. Chem. Phys., 16, 2843-2862, doi:10.5194/acp-16-2843-2016,
2016

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