Poster's note: old but seemingly never published to list.  It's a
critical paper, so if you haven't read it, please do so.

http://keith.seas.harvard.edu/papers/127.Pierce.EfficientFormStratsAerosol.e.pdf

Efficient formation of stratospheric aerosol for climate engineering
by emission of condensible vapor from aircraft - 22 September 2010.

[1] Recent analysis suggests that the effectiveness of stratospheric
aerosol climate engineering through emission of nonā€condensable vapors
such as SO2 is limited because the slow conversion to H2SO4 tends to
produce aerosol particles that are too large; SO2 injection may be so
inefficient that it is difficult to counteract the radiative forcing
due to a CO2 doubling. Here we describe an alternate method in which
aerosol is formed rapidly in the plume following injection of H2SO4, a
condensable vapor, from an aircraft. This method gives better control
of particle size and can produce larger radiative forcing with lower
sulfur loadings than SO2 injection. Relative to SO2 injection, it may
reduce some of the adverse effects of geoengineering such as radiative
heating of the lower stratosphere. This method does not, however,
alter the fact that such a geoengineered radiative forcing can, at
best, only partially compensate for the climate changes produced by
CO2.

Citation: Pierce, J. R., D. K. Weisenstein, P. Heckendorn, T. Peter,
and D. W. Keith (2010), Efficient formation of stratospheric aerosol
for climate engineering by emission of condensible vapor from
aircraft, Geophys. Res. Lett., 37, L18805, doi:10.1029/2010GL043975.

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