http://iopscience.iop.org/article/10.1088/1748-9326/aa6de5

Environmental Research Letters <http://iopscience.iop.org/journal/1748-9326>
ACCEPTED MANUSCRIPT • OPEN ACCESS
Assessment of reasonable opportunities for direct air capture

Jennfer Wilcox1, Peter Psarras2 and Simona Liguori3

Accepted Manuscript online 19 April 2017 • ©2017 IOP Publishing Ltd

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Article information
<http://iopscience.iop.org/article/10.1088/1748-9326/aa6de5#>
Abstract

This work explores the possibility of using CO2 captured directly from the
atmosphere for several applications that require low to moderate purities.
Comparisons of the minimum and real work for separating CO2 from air,
natural gas combined cycle flue gas and pulverized coal combustion flue gas
are proposed and discussed. Though it is widely accepted that the
separation of CO2 from air to high purity is more energy-intensive than
separating CO2 from more concentrated sources, this study presents select
cases where the separation of CO2 from air to low and moderate purities is
energetically equivalent with the work required for flue gas CO2
separation. These energetically-competitive cases are shown to be dependent
on the percent capture and final CO2 purity desired. In particular, several
technologies can be considered as CO2 utilization opportunities in which
dilute CO2 may be an adequate feedstock. Specifically, this study is
focused on enhanced oil recovery and microalgae cultivation technologies,
which appear to be the most beneficial near-term applications for
utilization of CO2 from direct air capture

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