https://acp.copernicus.org/preprints/acp-2022-351/

*Authors*
Je-Yun Chun, Robert Wood, Peter Blossey, and Sarah J. Doherty

*Received: 19 May 2022 *
*Discussion started: 30 May 2022*

*Abstract*
Ship tracks in subtropical *marine low clouds are simulated and
investigated using large eddy simulations.* Five variants of a shallow
subtropical stratocumulus-topped marine boundary layer (MBL) are chosen to
span a range of background aerosol concentrations and variations in
free-tropospheric (FT) moisture. Idealized time-invariant meteorological
forcings and approximately steady-state aerosol concentrations constitute
the background conditions. We *investigate processes controlling cloud
microphysical, macrophysical and radiative responses to aerosol injections.*
For the analysis, we use novel methods to decompose the liquid water path
(LWP) adjustment into changes in cloud properties, and the cloud radiative
effect (CRE) into contributions by cloud macro- and microphysics. The key
results are that (a) the cloud top entrainment rate increases in all cases,
with stronger increases for thicker than thinner clouds; (b) the drying and
warming induced by increased entrainment is offset to differing degrees by
corresponding responses in surface fluxes, precipitation and radiation; (c)
MBL turbulence responds to changes caused by the aerosol perturbation, and
this significantly affects cloud macrophysics; (d) across two days'
simulation, clouds were brightened in all cases. In a pristine MBL,
significant drizzle suppression by aerosol injections results not only in
greater water retention, but also in turbulence intensification, leading to
a significant increase in cloud amount. In this case, Twomey brightening is
strongly augmented by an increase in cloud thickness and cover. In
addition, a reduction in the loss of aerosol through coalescence scavenging
more than offsets the entrainment dilution. This interplay precludes
estimation of the lifetime of the aerosol perturbation. *The combined
responses of cloud macro- and microphysics lead to 10–100 times more
effective cloud brightening in these cases relative to those in the
non-precipitating MBL cases. *In moderate and polluted MBLs entrainment
enhancement makes the boundary layer drier, warmer and more stratified,
leading to a decrease in cloud thickness. Counterintuitively, this LWP
response offsets the greatest fraction of the Twomey brightening in a
moderately moist free troposphere. This finding differs from previous
studies which found larger offsets in a drier free troposphere, and results
from a greater entrainment enhancement in initially thicker clouds, so the
offsetting effects are weaker. The injected aerosol lifetime in cases with
polluted MBLs is estimated as 2–3 days, which is longer than the estimates
from satellite images.

*Source: European Geosciences Union *

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