https://www.sciencedirect.com/science/article/pii/S1674927823000357

*Authors*
Xiao-Yu Jin, Long Cao

*20 March 2023*

https://doi.org/10.1016/j.accre.2023.03.002

*Abstract*
*Carbon dioxide removal* and *solar radiation modification (SRM)* are two
classes of proposed climate intervention methods. A thorough understanding
of climate system response to these methods calls for a good understanding
of the carbon cycle response. In this study, we used an Earth system model
to examine the response of global climate and carbon cycle to artificial
ocean alkalinization (AOA), a method of CO2 removal, and reduction in solar
irradiance that represents the overall effect of solar radiation
modification. In our simulations, AOA is applied uniformly over the global
ice-free ocean under the RCP8.5 scenario to bring down atmospheric CO2 to
the level of RCP4.5, and SRM is applied uniformly over the globe under the
RCP8.5 scenario to bring down global mean surface temperature to the level
of RCP4.5. Our simulations show that with the same goal of temperature
stabilization, AOA and SRM cause fundamentally different perturbations of
the ocean and land carbon cycle. By the end of the 21st century, relative
to the simulation of RCP8.5, AOA-induced changes in ocean carbonate
chemistry enhances global oceanic CO2 uptake by 983 PgC and increases
global mean surface ocean pH by 0.42. Meanwhile, AOA reduces land CO2
uptake by 79 PgC and reduces atmospheric CO2 concentration by 426 × 10−6.
By contrast, relative to the simulation of RCP8.5, SRM has a minor effect
on the oceanic CO2 uptake and ocean acidification. SRM-induced cooling
enhances land CO2 uptake by 140 PgC and reduces atmospheric CO2
concentration by 63 × 10−6. A sudden termination of SRM causes a rate of
temperature change that is much larger than that of RCP8.5. A sudden
termination of AOA causes a rate of temperature change that is comparable
to that of RCP8.5 and a rate of ocean acidification that is much larger
than that of RCP8.5.

*Keywords*
Carbon dioxide removal, Solar radiation modification, Geoengineering,
Carbon cycle, Ocean acidification

*Source: ScienceDirect*

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