https://acp.copernicus.org/articles/23/9725/2023/

*Authors*
Felix Wrana <[email protected]>, Ulrike Niemeier, Larry W.
Thomason, Sandra Wallis, and Christian von Savigny
*Citations*: Wrana, F., Niemeier, U., Thomason, L. W., Wallis, S., and von
Savigny, C.: Stratospheric aerosol size reduction after volcanic eruptions,
Atmos. Chem. Phys., 23, 9725–9743, https://doi.org/10.5194/acp-23-9725-2023,
2023.

Received: 26 Apr 2023 – Discussion started: 04 May 2023 – Revised: 18 Jul
2023 – Accepted: 24 Jul 2023 – *Published: 01 Sep 2023*
*Abstract*

The stratospheric aerosol layer plays an important role in the radiative
balance of Earth primarily through scattering of solar radiation. The
magnitude of this effect depends critically on the size distribution of the
aerosol. The aerosol layer is in large part fed by volcanic eruptions
strong enough to inject gaseous sulfur species into the stratosphere. The
evolution of the stratospheric aerosol size after volcanic eruptions is
currently one of the biggest uncertainties in stratospheric aerosol
science. We retrieved aerosol particle size information from satellite
solar occultation measurements from the Stratospheric Aerosol and Gas
Experiment III mounted on the International Space Station (SAGE III/ISS)
using a robust spectral method. We show that, surprisingly, some volcanic
eruptions can lead to a decrease in average aerosol size, like the 2018
Ambae and the 2021 La Soufrière eruptions. In 2019 an intriguing contrast
is observed, where the Raikoke eruption (48∘ N, 153∘ E) in 2019 led to the
more expected stratospheric aerosol size increase, while the Ulawun
eruptions (5∘ S, 151∘ E), which followed shortly after, again resulted in a
reduction in the values of the median radius and absolute distribution
width in the lowermost stratosphere. In addition, the Raikoke and Ulawun
eruptions were simulated with the aerosol climate model MAECHAM5-HAM. In
these model runs, the evolution of the extinction coefficient as well as of
the effective radius could be reproduced well for the first 3 months of
volcanic activity. However, the long lifetime of the very small aerosol
sizes of many months observed in the satellite retrieval data could not be
reproduced.
*Source: European Geosciences Union*

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