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https://www.pnas.org/doi/10.1073/pnas.2221810120

*Authors*
Andrea Burke <https://www.pnas.org/doi/10.1073/pnas.2221810120#con1>
https://orcid.org/0000-0002-3754-1498 [email protected], Helen M. Innes
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con2>
https://orcid.org/0000-0002-4003-3910, Laura Crick
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con3>, Kevin
J. Anchukaitis <https://www.pnas.org/doi/10.1073/pnas.2221810120#con4>, Michael
P. Byrne <https://www.pnas.org/doi/10.1073/pnas.2221810120#con5>
https://orcid.org/0000-0001-9019-3915, William Hutchison
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con6>, Joseph R. McConnell
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con7>
https://orcid.org/0000-0001-9051-5240, Kathryn A. Moore
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con8>
https://orcid.org/0000-0002-9242-5422, James W. B. Rae
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con9>
https://orcid.org/0000-0003-3904-2526, Michael Sigl
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con10>
https://orcid.org/0000-0002-9028-9703, and Rob Wilson
<https://www.pnas.org/doi/10.1073/pnas.2221810120#con11>

*06 November 2023*

https://doi.org/10.1073/pnas.2221810120

*Significance*
Stratospheric sulfate aerosols from large volcanic eruptions reflect
incoming sunlight and cool climate, but this process is not well quantified
due to a limited observational record. Here, we take advantage of the
unique sulfur isotope fingerprint imparted by UV radiation in the upper
stratosphere, measuring volcanic sulfate peaks in polar ice cores to
determine their climatically important stratospheric component. We find
evidence that several of the coldest decades in the last two thousand
years—linked with major climatic and societal disruption—were driven by a
relatively small amount of stratospheric sulfate from high-latitude
eruptions. This challenges the view that tropical eruptions have the
largest climatic impacts and suggests enhanced climatic sensitivity to
high-latitude volcanic forcing in the Northern Hemisphere.

*Abstract*
The 540s, 1450s, and 1600s represent three of the five coldest decades in
the Common Era (CE). In each of these cases, the cause of these cold pulses
has been attributed to large volcanic eruptions. However, the provenance of
the eruption and magnitude of the volcanic forcing remains uncertain. Here,
we use high-resolution sulfur isotopes in Greenland and Antarctic ice cores
measured across these events to provide a means of improving sulfur loading
estimates for these eruptions. In each case, the largest reconstructed
tree-ring cooling is associated with an extratropical eruption, and the
high-altitude stratospheric sulfate loading of these events is
substantially smaller than previous estimates (by up to a factor of two).
These results suggest an increased sensitivity of the reconstructed
Northern Hemisphere summer temperature response to extratropical eruptions.
This highlights the importance of climate feedbacks and processes that
amplify and prolong the cooling signal from high latitudes, such as changes
in sea ice extent and ocean heat content.

*Source: PNAS*

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