https://www.newswise.com/articles/washu-researchers-will-explore-stratospheric-aerosol-injection-with-a-1-5-million-grant-from-the-simons-foundation-international

*By Washington University in St. Louis*

*15 May 2024*

Newswise — Geoengineering, or large-scale manipulation of the climate by
humans, has spawned sci-fi treatments aplenty, from supervillains trying to
control the weather for their own ends to vivid imaginings of what future
catastrophes might result from unsustainable environmental control. Rajan
Chakrabarty <https://engineering.wustl.edu/faculty/Rajan-Chakrabarty.html>,
the Harold D. Jolley Career Development Associate Professor in the McKelvey
School of Engineering at Washington University in St. Louis, takes a more
nuanced view.

Chakrabarty and collaborators Rohan Mishra
<https://engineering.wustl.edu/faculty/Rohan-Mishra.html>, associate
professor of mechanical engineering & materials science, and Lu Xu
<https://engineering.wustl.edu/faculty/Lu-Xu.html>, assistant professor of
energy, environmental & chemical engineering, both in McKelvey Engineering,
won a three-year, $1.5 million grant from the Simons Foundation
International to explore potential candidates for a geoengineering
technology called stratospheric aerosol injection (SAI). SAI involves
seeding small particles or aerosols into the upper atmosphere to offset
global warming caused by human-made greenhouse gas emissions.

SAI is one pathway for humans to replicate the natural cooling effect
observed after the 1991 eruption of Mount Pinatubo, a volcano in the
Philippines. The eruption spewed 10-20 million tons of sulfate aerosols
into the stratosphere where those particles reflected enough sunlight to
cause a global temperature decrease of about half a degree Celsius in 1992.

Chakrabarty and Mishra have already worked together on analyzing the
chemical and optical properties of particles in wildfire smoke
<https://engineering.wustl.edu/news/2023/Fanning-the-Flames.html>,
revealing that wildfires have a much larger warming effect than climate
modelers thought. This new project would similarly inform climate
projections used in SAI and geoengineering more broadly. Chakrabarty says
models are currently missing key ingredients, including how particles that
might be injected into the atmosphere will interact with solar radiation
and ozone over time.

“Think about it like a dish you are preparing,” Chakrabarty said. “You have
to consider what ingredients you’re putting in, how much of each
ingredient, and how those ingredients will interact in the final meal. For
SAI, our ingredients are particles, and we need to know what are their
light scattering and absorption properties? What is their interaction with
ozone? What happens if there are manufacturing defects in individual
particles? These factors will all impact what happens when we put these
aerosols in the stratosphere.”

Combining Chakrabarty’s expertise in aerosol optics and modeling, Mishra’s
techniques for characterizing and optimizing material properties at the
atomic scale, and Xu’s expertise in atmospheric chemistry and chemical
kinetics, including ozone chemistry, the team will help scientists make
sure that if SAI is deployed, it is as effective and safe as possible. They
plan on compiling a database of optical and chemical properties for the
most promising aerosol candidates, including considerations of size,
composition, atmospheric interaction and aging processes. All these
features can be readily incorporated into climate models to accurately
assess the impacts of different SAI scenarios in modulating earth’s
temperature and the environment.

“Our ultimate goal is to help the scientific community work out the best
candidates for SAI geoengineering,” Chakrabarty said. “We’re using the
unique expertise we have here in McKelvey Engineering to explore the nitty
gritty details for top SAI candidates in terms of their material and
optical properties, safety considerations and how the particles behave over
time. Looking at these properties across bulk and atomic scales will
provide critical information for future users, including geoengineers,
climate modelers and aerosol manufacturers.”

This award is part of the Simons Foundation’s Mathematics and Physical
Sciences (MPS) division's Solar Radiation Management program (SRM).
Chakrabarty, Mishra and Xu will participate in Simons Foundation activities
along with fellow SRM awardees.
*Source: Newswise*

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