https://www.sciencedirect.com/science/article/pii/S295013852400007X

*Authors*
H.J. Rubin, C.-E. Yang, F.M. Hoffman, J.S. Fu

*01 August 2024*

https://doi.org/10.1016/j.gecadv.2024.100011

*Abstract*
Even with immediate implementation of global policies to mitigate carbon
dioxide emissions, the impacts of climate change will continue to worsen
over the next decades. One potential response is stratospheric aerosol
injection (SAI), where sulfur dioxide is released into the stratosphere to
block incoming solar radiation. SAI does not reduce the level of carbon
dioxide in the atmosphere, but it can slow warming and act as a stopgap
measure to give the world more time to pursue effective carbon reduction
strategies. While SAI is controversial, it remains a technically feasible
proposition. It ought to be thoroughly modeled both to characterize global
risks better and to further the scientific community’s understanding of
stratospheric aerosol dynamics. SAI relies on sulfate aerosols which have a
lifetime of several years in the stratosphere but will eventually be
deposited back onto Earth’s surface. While sulfate is an important nutrient
for many ecosystems, high concentrations can cause acidification,
eutrophication, and biodiversity loss. We use model outputs from the
Geoengineering Model Intercomparison Project (GeoMIP) to track the impacts
of sulfur deposition from SAI to various ecoregions through comparison with
historical climate and future Shared Socioeconomic Pathway (SSP) scenarios.
Our results demonstrate that dry sulfur deposition will continue to decline
worldwide, regardless of scenario, from a high of 41 Tg S/yr in 1981 to
under 20 Tg S/yr by 2100. Wet sulfur deposition, however, is much more
uncertain and further work needs to be done in this area to harmonize model
estimates. Under SAI, many ecoregions will experience notably different
sulfur deposition regimes by the end of the century compared to historical
trends. In some places, this will not be substantially different than the
impacts of climate change under SSP2–4.5 or SSP5–8.5. However, in some
ecoregions the model projections disagree dramatically on the magnitude of
future trends in both emissions and deposition, with, for example,
UKESM1–0-LL projecting that SO42- deposition in deciduous needleleaf
forests under G6 Sulfur will reach 394 % of SSP2–4.5 deposition by the
2080 s while CESM2-WACCM projects that SO42- deposition will remain at
170 % of SSP2–4.5 deposition during that same time period. Our work
emphasizes the lack of agreement between models and the importance of
improving our understanding of SAI impacts for future climate
decision-making.

*Source: ScienceDirect *

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