https://essopenarchive.org/doi/pdf/10.22541/essoar.172374105.56686934

*Authors*
Qiurun Yu, Yi Huang

*15 August 2024*

*Abstract *
To facilitate the quantification of the stratospheric aerosol radiative
effect, this study generates a set of aerosol direct radiative effect
(ADRE) kernels based on MERRA-2 reanalysis data. These radiative kernels
measure the sensitivities of ADRE to perturbations in scattering and
absorbing aerosol optical depth (AOD), respectively. Both broadband and
band-by-band radiative kernels are developed to account for the wavelength
dependency of ADRE. The broadband kernels are then emulated by a
multivariate regression model, which predicts the kernel values from a
handful of predictors, including the top-of-atmosphere (TOA) insolation,
TOA reflectance, and stratospheric AOD. These kernels offer an efficient
and versatile way to assess the ADRE of stratospheric aerosols. The ADREs
of the 2022 Hunga volcano eruption and the 2020 Australia wildfire are
estimated from the kernels and validated against radiative transfer
model-calculated results. The Hunga eruption induced a global mean cooling
forcing of -0.46 W/m² throughout 2022, while the Australia wildfire caused
a warming forcing of +0.28 W/m² from January to August. The kernel
estimation can capture over 90% of the ADRE variance with relative error
within 10%, in these assessments. The results demonstrate the spectral
dependencies of stratospheric ADRE and highlight the distinct radiative
sensitivity of stratospheric aerosols, which differs significantly from
that of tropospheric aerosols.

*Plain Language Summary *
Stratospheric aerosols influence the Earth's energy balance by scattering
and absorbing solar radiation, making it crucial to accurately measure
their radiative impact. However, quantifying the aerosol radiative impact
is computationally expensive if using radiative transfer models. In this
work, we develop a set of aerosol radiative kernels, which can provide a
flexible and efficient means for calculating the radiative effects of
stratospheric aerosols. The kernels have been demonstrated to effectively
quantify the radiative impacts of stratospheric aerosols resulting from
wildfire and volcanic eruption events.

*Source: ESS OPEN ARCHIVE *

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