https://agupubs.onlinelibrary.wiley.com/doi/full/10.1029/2024GL113718

*Authors*
Fan Liu, Feiyue Mao, Daniel Rosenfeld, Zengxin Pan, Lin Zang, Yannian Zhu,
Wei Gong

First published: *01 April 2025*

https://doi.org/10.1029/2024GL113718

*Abstract*
The idea of cooling the Earth by marine cloud brightening is well
established. All prior studies considered enhancing cloud albedo only with
fine aerosols (FA). Adding coarse sea spray aerosols (CSA, radius>1 μm) has
been thought to have the opposite effect. Using nearly a decade of
satellite observations and global aerosol reanalysis, we found that the
maximum radiative cooling effect from marine stratocumulus occurs when FA
is around 3 μg m−3 and CSA is around 30 μg m−3. Under low winds and high
stability conditions, optimal FA and CSA can enhance cooling by −95 W m−2,
nearly 60% more than adding FA alone. This CRE response to FA and CSA was
consistently observed across various cloud-controlling factors, thus
minimizing the probability of being caused by meteorological
co-variability. These findings improve our understanding of how different
aerosols affect Earth's climate, improve the evaluation of cooling achieved
through marine cloud brightening, and support its feasibility.

*Key Points*
Maximum cooling of marine stratocumulus occurs at about 3 μg m−3 of fine
aerosols and 30 μg m−3 of coarse sea salt

Optimal fine and coarse sea salt aerosol is associated with up to −95 W m−2
more cloud cooling than in the clean condition

Observational evidence eliminates concerns about the previously assumed
warming effect of coarse sea salt in marine cloud brightening

*Plain Language Summary*
Geoengineering aims to cool the Earth by artificially injecting aerosols
into marine stratocumulus clouds over the oceans by flight or ship, called
marine cloud brightening (MCB). Previous studies mainly focused on the
cooling effects of fine aerosols (FA), while coarse sea salt aerosols (CSA,
radius >1 μm) were thought to cause warming. Due to technical limitations,
CSA is unintentionally introduced during sea spray injection in MCB
project. This raises concerns about the feasibility of MCB using only fine
sea spray, as it's difficult to avoid the tail of large spray drops.
However, by analyzing nearly 10 years of satellite observations and global
aerosol reanalysis, we found that the largest cooling effect of marine
stratocumulus clouds is associated with FA of about 3 μg m−3 and CSA of
around 30 μg m−3. This optimal combination yields a 60% greater radiative
cooling enhancement than optimal FA can achieve alone. The scheme of
injecting CSA at MCB project appears as an advantage rather than a
limitation and makes MCB closer to practical.

*Source: AGU*

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