https://egusphere.copernicus.org/preprints/2026/egusphere-2026-444/

*Authors: *Andrin Jörimann, Timofei Sukhodolov, Simone Tilmes, David
Plummer, Shingo Watanabe, Hideharu Akiyoshi, Gabriel Chiodo, Daniele
Visioni, Sandro Vattioni, Eugene Rozanov, Ewa M. Bednarz, Béatrice Jossé,
Yousuke Yamashita, and Thomas Peter

*04 February 2026*

*Abstract*
Stratospheric aerosol injection (SAI) could slow surface warming and help
prevent some irreversible tipping points in the climate system. However,
potential side effects include changes in stratospheric ozone and warming
due to infrared ab sorption by the aerosol, which can alter surface
ultraviolet radiation, hydrology, and weather through
stratosphere-troposphere coupling. Previous multi-model studies have
reported large model discrepancies regarding these effects. Here we present
results from an experiment within the Chemistry-Climate Model Initiative
Phase 2 (CCMI-2022), designed to constrain inter-model uncertainties by
applying a common stratospheric aerosol forcing to five chemistry-climate
models using an SAI scenario offsetting all surface warming after 2025 in a
moderate greenhouse gas emission scenario. All models show a global total
column ozone decrease in the first three decades of no more than ∼10 DU
relative to a no-SAI case. Despite sizable differences in stratospheric
heating, the models yield a qualitatively similar pattern of ozone
redistribution. Changes in key processes, such as the ClOx activation and
NOx passivation, and the strengthening of the deep branch of the
Brewer-Dobson circulation, are widely robust across all models, though
their relative importance and contribution to ozone changes varies
considerably. In three of the models, we separate chemical and dynamical
contributions, and find significant nonlinearities from feedbacks between
chemistry and dynamics, highlighting where model development and
sensitivity experiments are most needed to advance the understanding of the
middle atmosphere in future mitigation scenarios involving SAI.

*Source: EGUsphere *

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