I am facing same issue while re-connecting to my TunnelBear VPN. TunnelBear VPN 
uses open-vpn service. I have configured VPN as per instructions by TunnelBear. 
And it works fine when connect first time, but after that when choose "Turn 
Off" from Netowrok-Manager then choose "Connect" again, then I see this same 
error. See snapshot from syslog:
Dec 17 20:45:25 KUMAR-PC NetworkManager[902]: <info>  [1576611925.5171] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN plugin: state changed: starting (3)
Dec 17 20:45:25 KUMAR-PC NetworkManager[902]: <info>  [1576611925.5172] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN connection: (ConnectInteractive) reply received
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: WARNING: --keysize is DEPRECATED and 
will be removed in OpenVPN 2.6
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: OpenVPN 2.4.4 x86_64-pc-linux-gnu 
[SSL (OpenSSL)] [LZO] [LZ4] [EPOLL] [PKCS11] [MH/PKTINFO] [AEAD] built on May 
14 2019
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: library versions: OpenSSL 1.1.1  11 
Sep 2018, LZO 2.08
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: WARNING: --ns-cert-type is 
DEPRECATED.  Use --remote-cert-tls instead.
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: NOTE: the current --script-security 
setting may allow this configuration to call user-defined scripts
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: TCP/UDP: Preserving recently used 
remote address: [AF_INET]103.228.153.233:443
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: UDP link local: (not bound)
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: UDP link remote: 
[AF_INET]103.228.153.233:443
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: NOTE: chroot will be delayed because 
of --client, --pull, or --up-delay
Dec 17 20:45:25 KUMAR-PC nm-openvpn[6237]: NOTE: UID/GID downgrade will be 
delayed because of --client, --pull, or --up-delay
Dec 17 20:45:27 KUMAR-PC nm-openvpn[6237]: [9563/server] Peer Connection 
Initiated with [AF_INET]103.228.153.233:443
Dec 17 20:45:28 KUMAR-PC nm-openvpn[6237]: Option 'explicit-exit-notify' in 
[PUSH-OPTIONS]:3 is ignored by previous <connection> blocks
Dec 17 20:45:28 KUMAR-PC nm-openvpn[6237]: Note: option tun-ipv6 is ignored 
because modern operating systems do not need special IPv6 tun handling anymore.
Dec 17 20:45:28 KUMAR-PC nm-openvpn[6237]: ERROR: Cannot ioctl TUNSETIFF tun0: 
Device or resource busy (errno=16)
Dec 17 20:45:28 KUMAR-PC nm-openvpn[6237]: Exiting due to fatal error
Dec 17 20:45:28 KUMAR-PC NetworkManager[902]: <warn>  [1576611928.9900] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN plugin: failed: connect-failed (1)
Dec 17 20:45:28 KUMAR-PC NetworkManager[902]: <warn>  [1576611928.9901] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN plugin: failed: connect-failed (1)
Dec 17 20:45:28 KUMAR-PC NetworkManager[902]: <info>  [1576611928.9902] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN plugin: state changed: stopping (5)
Dec 17 20:45:28 KUMAR-PC NetworkManager[902]: <info>  [1576611928.9903] 
vpn-connection[0x5568a73e41c0,d79431f3-7dda-41cb-b74b-e7b71ed48592,"TunnelBear 
India",0]: VPN plugin: state changed: stopped (6)

If someone needs, then I can reproduce this with additional traces. But as much 
I could learn from this problem is that, while "Turn Off" from Netowrk-Manager, 
Network-Manager is not able to stop openvpn process.
If I stop this openvpn process manually, then try to "Connect" from 
Network-Manager menu, it works fine.

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Packages, which is subscribed to linux in Ubuntu.
https://bugs.launchpad.net/bugs/1767322

Title:
  "Activation of network connection failed" popup shows incessantly

Status in linux package in Ubuntu:
  Confirmed
Status in network-manager package in Ubuntu:
  Confirmed

Bug description:
  All network connections work normally, however the popup "Activation
  of network connection failed" keeps showing.

  ProblemType: Bug
  DistroRelease: Ubuntu 18.04
  Package: network-manager 1.10.6-2ubuntu1
  ProcVersionSignature: Ubuntu 4.15.0-20.21-lowlatency 4.15.17
  Uname: Linux 4.15.0-20-lowlatency x86_64
  ApportVersion: 2.20.9-0ubuntu7
  Architecture: amd64
  CurrentDesktop: ubuntu:GNOME
  Date: Fri Apr 27 20:04:56 2018
  IfupdownConfig:
   # interfaces(5) file used by ifup(8) and ifdown(8)
   auto lo
   iface lo inet loopback
  InstallationDate: Installed on 2018-04-03 (24 days ago)
  InstallationMedia: Ubuntu 18.04 LTS "Bionic Beaver" - Alpha amd64 (20180402)
  IpRoute:
   default via 192.168.1.1 dev wlp2s0 proto dhcp metric 600 
   169.254.0.0/16 dev virbr1 scope link metric 1000 linkdown 
   192.168.1.0/24 dev wlp2s0 proto kernel scope link src 192.168.1.128 metric 
600 
   192.168.100.0/24 dev virbr1 proto kernel scope link src 192.168.100.1 
linkdown 
   192.168.122.0/24 dev virbr0 proto kernel scope link src 192.168.122.1 
linkdown
  NetworkManager.state:
   [main]
   NetworkingEnabled=true
   WirelessEnabled=true
   WWANEnabled=true
  SourcePackage: network-manager
  UpgradeStatus: No upgrade log present (probably fresh install)
  nmcli-nm:
   RUNNING  VERSION  STATE      STARTUP  CONNECTIVITY  NETWORKING  WIFI-HW  
WIFI     WWAN-HW  WWAN    
   running  1.10.6   connected  started  full          enabled     enabled  
enabled  enabled  enabled

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