Milan Regec schrieb:

I am convinced that LyX/LaTeX output looks quite nice,
however so far all the PDFs I've seen created by these tools
were--behind the scenes--at best junky.

Is there a way LyX+LaTeX can produce tagged PDF that will
eventually be reflowable and sport accessibility features?
or bookmars generated from TOC/styles?

Have a look at the "pdftex" project if a nd how tagged PDFs are supported. It is recommended to produce PDFS out if LyX by using the menu Export->PDF(pdflatex). pdflatex uses pdftex.

Having PDFS with automatically created bookmarks, interlinks for cross-references, hyperlinks for URLS, and PDF-file descriptions like the author name etc. is very easy: Use the LaTeX-package "hyperref" in the preamble.
Here you find more about this:
http://www.tug.org/applications/hyperref/manual.html

You can also have a lookt at the document preamble of
http://wiki.lyx.org/uploads/LyX/LyXMathebefehle/LyXMathebefehle-3-08.lyx
to see how hyperref is used to get all this. The PDF output looks like:
http://wiki.lyx.org/uploads/LyX/LyXMathebefehle/LyXMathebefehle-3-08.pdf

regards Uwe

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