Apple - Support - Discussions - iPod cannot be synced. Required folder ...

USB hub used? try with out
There is also another preference fix in the above link.

also found this:
to fix the iphone / ipod cannot be synced. The missing file cannot be found, 
simply do the folowing.

1) close iphoto and itunes
2) find the iphoto library in finder, most probably located in your users 
folder under pictures.
3) right click on iphoto library (might be named diferently) and choose show 
package contents
4) delete the folder caches and ipod photo cache.
5) restart iphoto 
6) restart itunes
if itunes asks that the library is linked with another ipod, say yes to the 
warning to re sync with your ipod/ iphone
On Jan 26, 2010, at 3:03 PM, Harry Jacobson-Beyer wrote:

> Hi Happy New Year to all!
> 
> I'm having problems with my iPod since I upgraded to leopard 5 or 6
> months ago.
> 
> My music library has duplicate titles for most songs.
> 
> Most of my songs have been deleted from my iPod.
> 
> Also when I attempt to sync my Ipod I get the following message:
> 
> The iPod "Harry Jacobson-Beyer's iPod" cannot be synced. A file was
> specified instead of a folder.
> 
> Any help will be appreciated.
> 
> Thanks.
> 
> Harry
> 
> 
> 
> 
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