The biggest challenge is designing a high-efficiency DC-DC converter for 
the tubes; it is the primary consumer of energy. Generally, you will get 
higher efficiency at higher battery voltage. 

Next, you will need to determine the battery size/voltage/capacity. I 
gathered a lot of data about various storage technologies (NiCd, Li-ion, 
NiMH, lead-acid, supercapacitors). Conclusion is what I expected: Li-ion. 
There are all sorts of Li-ion cells in various size, shape, capacity for 
phones, tablets, and laptops. Li-ion also has the simplest charging 
algorithm *as long as you dont fast-charge*. 

If you just want a portable clock, I'd start with Li-ion battery-packs for 
power tools. Then you can just use the existing charger.

I'm working on a dynamotor portable nixie clock, and it will use a sealed 
lead-acid (SLA) battery. Heavy, noisy, but very cool.

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