Artificial leaf converts water into fuel
Friday, 30 September 2011
 
by Phillip English
_Cosmos Online_ 
(http://www.cosmosmagazine.com/news/4802/www.cosmosmagazine.com)  

 
 
SYDNEY: Drawing inspiration from leaves and photosynthesis, two separate  
research teams have successfully demonstrated improved techniques to convert  
carbon dioxide and water into usable fuels.  
A pair of papers, published today in the journal Science, describe two  
different approaches to generating fuel: one involving an artificial leaf that  
can split water molecules to create hydrogen fuel, the other aimed at 
recycling  carbon dioxide. 
The first study, a combined effort of researchers from the University of  
Illinois and U.S.-based company Dioxide Materials, details a more efficient  
method of reducing carbon dioxide (CO2) to carbon monoxide (CO), a component 
of  synthetic gas fuels. 
"Our approach is called artificial photosynthesis. We collect solar energy  
like plant life collects solar energy, and then use that energy to convert 
the  CO2 into either petrol or some other useful product," said co-author on 
the fist  paper Richard Masel, a researcher from Dioxide Materials. 
"We were hoping to get 50% energy efficiency but we actually observed over  
80%. That makes CO2 recycling feasible," he said.  
Recapturing carbon versus recycling 
The capture and storage of carbon dioxide produced from fossil fuel 
emissions  has become a prominent issue as a result of concerns about global 
climate  change.  
Some examples of storage methods involve the sequestering of carbon dioxide 
 in minerals, or pumping the gas into vacated geological formations such as 
oil  or gas fields. But another option is to try and recycle this gas.  
"My view is that burying the CO2 and leaving it for future generations is 
not  a solution to the problem. Instead we need to find ways to recycle CO2 
into  something useful," said Masel.  
To do this, his team has focussed on a technique that will enable the gas 
to  be recycled - broken down into its original components, and converted 
into fuel.  
Improved catalyst changes the game 
The concept of using electricity to reduce CO2 is not new, but in previous  
experiments, high voltages had to be used to overcome the energy of the 
chemical  bonds in carbon dioxide before it could be broken down into oxygen 
and carbon  monoxide.  
To get around this, researchers can introduce a catalyst - a substance that 
 accelerates a chemical reaction without itself being affected. This 
induces an  alternative reaction that needs significantly less energy, and 
therefore less  voltage, to break down the carbon dioxide into useful fuel. 
In the case of the current study, the researchers discovered that a  
particular chemical compound known as "EMIM-BF4" was a very efficient catalyst  
in 
breaking down carbon dioxide.  
Highly accessible technology 
One of the benefits of the technology is its ability to be plugged into any 
 external energy source such as a wind farm or solar cell array.  
The proposed device would then take in the energy, CO2 and water and 
produce  synthetic gas. This synthetic gas could then be used directly in 
industrial  processes or sent to a refinery to make petrol, researchers 
explained. 
"I think that is a very exciting finding. Lowering the energy requirement 
for  the conversion of CO2 into CO is vital if CO2 is to be efficiently 
transformed  into fuels and other carbon based products," said Leone Spiccia, a 
chemist from  Monash University in Melbourne.  
"The approach is complementary to efforts to split water into oxygen and  
hydrogen fuel. Whilst both approaches have great merit, an advantage of  
converting CO2 into fuels is that existing engines and distribution  
infrastructures can be used." 
A green alternative 
Meanwhile, an effort between American and Dutch industrial researchers has  
shown that it is possible to use solar energy to split water with cheaper  
materials than previously thought. 
The focus of the second paper to be published in Science is a single  
device capable of splitting water into oxygen and hydrogen gases by directly  
harnessing solar energy - an 'artificial' leaf.

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