Quoting Sung-Ho KIM <[EMAIL PROTECTED]>:

> Hi, All,
> 1) According to A. David Rae��s paper, Acta Cryst.
> (1990), B46, 474-487, B1a1 can be transformed to P1c1
> using new axes (a+c)/2, b, c and origin relocated to
> put the glide at y=0." Please help me to convert B1a1
> (non-standard setting) into P1c1 (standard setting).
> In particular, how to convert atomic coordinate?
> 
> 2) If an atom (a1) partly occupy four different sites
> (b1, b2, b3 and b4) and the total amount of a1 have to
> keep 1.0, how to define constraints for a1 and b1~ b4
> atoms in GSAS? 
> Please give me an advice about two things.
> 

I may at least bring an answer to the second question. This topics has already 
been discussed in this list. The problem is a bit tricky but can be solved 
unambiguously.

 - if two atoms A and B (one of them may be vacancy) are distributed among 4 
sites 1, 2, 3, 4
 - if the total amount of A and B is known
 - if the diffraction contrast between A and B is sufficient

Then one may introduce the atoms as follows:
site 1:         A1 B1
site 2:         A2 B2
site 3:         A3 B3
site 4:         A4 B4 A'4 B'4 A''4 B''4

That means that two additional A and two additional B atoms are introduced on 
site 4.

The initial total amount of A and B should match the known composition.
Then, the constraints should be introduced as follows, where d represents the 
shifts on occupancy parameters expressed in number of atoms (that means that a 
multiplicative factor should be introduced in GSAS because this program deals 
with site fraction contrary to Fullprof):
dA1=-dB1=-dA4=dB4
dA2=-dB2=-dA'4=dB'4
dA3=-dB3=-dA''4=dB4
so that the A atoms removed from site 1 are compensated by B atoms in the same 
site and are transfered to site 4, and so on.

The procedure can be extended whatever the number sites. 

A brief explanation can be found in J.-M. Joubert, R. Cern�, M. Latroche, A. 
Percheron-Gu�gan and K. Yvon, "Site occupancies in LaNi5 three-substituted 
compound determined by means of multiwavelength X-ray powder diffraction." J. 
Appl. Crystallogr., 31 (1998) 327-332. The problem was a little bit different 
since it was about the determination of the distribution of 4 atoms among 2 
sites, but the solution is the same.

Best regards
Jean-Marc Joubert





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