Hi,

If an insulator is irradiated, free electrons should be created within it that 
are not free to recombine with the ions,
because they can't travel through an insulator. However they may attach 
themselves to other atoms. 
It might then be possible to magnetize this material, during which process the 
magnetic fields of the freed electrons
align with one another. Unpaired electrons in the ions created by the radiation 
may also contribute to the magnetic
field.

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