Hello, Arnold,

I replaced my current regulation circuit with a Thevenin
element with the Thevenin resistance matching load
resistance, with the idea of doing wheatstone bridge-type
potentiometry later on. The rheostat proved so convenient
to set the scale of the microammeter, I decided to
stick with current limitation instead of current regulation.
The latter may give more uniformity in particulate size,
but who knows whether size uniformity is better or worse
for product potency? Keeping the current low (<500 uA)
keeps the size range low anyway.

As you note, there is a trade-off. Current regulation makes
a more uniform product. But current limitation makes
transients measurable that may help elucidate processes
occurring at the electrodes. I like the latter feature more
because it is more of a research-grade circuit.
There is a relatively new research method called
Electrochemical Impedance Spectroscopy (abbreviated
EIS, by coincidence) that is used to investigate
electrolytic phenomena, especially corrosion phenomena,
based on frequency response ranging from 1 millihertz
to 100 kilohertz, which includes audible tones.
Sophisticated analysis of the noise-laden current leads
to equivalent RLC circuits that reveal quite a bit about
what's happening at and near the electrodes. Ordinary
people cannot afford the specialized apparatus used
for Electrochemical Impedance Spectroscopy, but the
human ear is a marvelous instrument and maybe could
detect a lot. Noisy signals can contain a large amount
of useful information - a good example is "star static,"
the nuisance RFI that became Radio Astronomy.

Best regards,

Matthew