I would create a new iTunes library (to avoid confusion and contamination). Hold down alt when you start iTunes, save the new library to the HDD, make sure it's saving ripped files to a location on that. Then sync the iPod with that library.

Managing multiple file locations within the same library is - to use a technical term - a really bad idea. Keep 'em separate.

To open a particular library either hold down alt on launch and navigate to it, or double click on the library file in the Finder. If you detach the HDD after quitting iTunes, it will want to know which library to use when next launched; point it at your usualone and it will default to that henceforth.
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On 10 Oct 2014, at 14:01, mac98aop wrote:

I don't want to copy them on to my Mac, but wonder if I can put them on an HDD, and then tell iTunes to find them AND make a playlist to put them on
an old iPod we use solely in the car.

Can I do that without confusing iTunes etc?

If so, any tips and step-by-steps gratefully received about how to burn CDs to the HDD, and then point the iPod and iTunes to that folder and not my
main one (without mucking up current setup with all iPods and iPhones
syncing to the main library).

Just seemed like a fun way of introducing the children to some much loved
'classics' on longer journeys, without clogging my MBP!

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