Dear all,

Anyone used Thermo Fisher's PD to identify phosphopeptides? I recently ran 
a phosphopeptide sample enriched by TiO2. The Mass spect is Orbitrap Velos, 
MS1 the FT at 30K resolution, MS2 the ion trap CID fragmentation. Although 
nearly every spectrum had a clear-cut feature of neutral loss of phosphoric 
acid, the identification was far from satisfactory. As many as 6,000 
phosphopeptides were identified in a single run, 4500 of them did not pass 
the peptide confidence threshold (low or medium confidence). When I look at 
QC identification results (e.g., E.coli digests, etc.), 80% of peptides 
were of high confidence.

I am not sure why the peptide confidence was so low when it comes to 
phosphopeptide identification in PD? Has any one of you encountered a 
similar problem? How did you configure the software, or just use HCD to run 
the sample again?

Best,

Siyuan

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