I am running PTMProphet (TPP v5.2.1-dev Flammagenitus, Build 
202003100907-8034) on MSFragger (MSFragger version MSFragger-2.3) output 
and ending up with strange results in specific cases.

For example, for a specific PSM, 52782, MSFragger outputs:

<spectrum_query start_scan="52782" 
uncalibrated_precursor_neutral_mass="2288.8486" assumed_charge="3" 
spectrum="QEP2_2018_0812_AZ_033_az736_AZ.52782.52782.3" end_scan="52782" 
index="41840" precursor_neutral_mass="2288.8384" 
retention_time_sec="6104.521">
<search_result>
<search_hit peptide="RYKAAFTECCQAADK" massdiff="471.0195" 
calc_neutral_pep_mass="1817.8188" peptide_next_aa="A" 
num_missed_cleavages="2" num_tol_term="2" num_tot_proteins="5" 
tot_num_ions="56" hit_rank="1" num_matched_ions="23" 
protein="sp|P02768|ALBU_HUMAN Serum albumin OS=Homo sapiens GN=ALB PE=1 
SV=2" peptide_prev_aa="K" is_rejected="0">
<modification_info>
<mod_aminoacid_mass mass="160.0307" position="9"/>
<mod_aminoacid_mass mass="160.0307" position="10"/>
</modification_info>
<search_score name="hyperscore" value="44.421"/>
<search_score name="nextscore" value="12.357"/>
<search_score name="expect" value="4.415e-15"/>
</search_hit>
</search_result>
</spectrum_query>

This would indicate that C9 is +57, C10 is +57 and there is an additional 
unlocalized mass diff of +471.

After running TPP I end up with output like this in interact.ipro.pep.xml 
for that scan:

<spectrum_query start_scan="52782" 
uncalibrated_precursor_neutral_mass="2288.8486" assumed_charge="3" 
spectrum="QEP2_2018_0812_AZ_033_az736_AZ.52782.52782.3" end_scan="52782" 
index="36796" precursor_neutral_mass="2288.8384" 
retention_time_sec="6104.521">
<search_result>
<search_hit peptide="RYKAAFTECCQAADK" massdiff="471.0195" 
calc_neutral_pep_mass="1817.8188" peptide_next_aa="A" 
num_missed_cleavages="1" num_tol_term="2" num_tot_proteins="5" 
tot_num_ions="56" hit_rank="1" num_matched_ions="23" 
protein="sp|P02768|ALBU_HUMAN" peptide_prev_aa="K" is_rejected="0" 
protein_descr="Serum albumin OS=Homo sapiens GN=ALB PE=1 SV=2">
<modification_info modified_peptide="RYKAAF[618]TEC[160]C[160]QAADK">
<mod_aminoacid_mass position="6" mass="618.0879"/>
<mod_aminoacid_mass position="9" mass="574.0287"/>
<mod_aminoacid_mass position="10" mass="574.0287"/>
</modification_info>.......

So it seems to me that we now have a modification mass addition of +471 on 
residues 6 9 and 10 rather than a mass addition of +471 on residue 6 and 
then an addition of +57 on residues 9 and 10.

In cases where there is just a mass diff (open modification) and no defined 
variable modifications output is as expected. This situation seems to occur 
when both defined variable modifications and open modifications are present.

I have confirmed the same behavior in older versions of MSFragger and TPP.

Any ideas would be much appreciated!
Thanks,
Alex

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