Silicone does work nicely on the larger cubes, but don't use a lot.  
Also I think it's better to work in the cube for a while without any 
lube to wear it down a little more smoothly first.  Once the larger 
cubes wear down from use they start popping (think explosion) so you 
want to try to delay that process as long as possible.

I use a small amount of lube in the larger cubes, but you have to 
apply it a little more often than for a 3x3x3.  I'd say I lube the 4x4 
once every two weeks or so, and I tend to lube the 3x3 about once 
every 3-4 weeks.

Hope that helps,
Chris

--- In [email protected], "jacben13" 
<[EMAIL PROTECTED]> wrote:
>
> Hello, I have just started speedcubing since I got my cube at
> Christmas, I am loving it.  In addition to the 3x3x3 cube I received,
> I have also gotten a 4x4x4 cube.  However, it does not turn nearly as
> nicely as by regular cube.  I have silicon spray, which worked great
> on the smaller cube, but I am wondering, will the lubricant make the
> larger cube too loose?  I understand that these cubes are looser to
> begin with, but I am wondering what people do to make them turn 
nicer.
>






 
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