I notice that the problem happens because LibreOffice shows splash
window first.

And I can suggest you some tricks to avoid this.
Just add --nologo parameter into the application's run command 
(Exec=libreoffice --nologo ...) in each file named 
/usr/share/applications/libreoffice-*.desktop, and stop to keep launchers on 
Unity panel. Splash window won't be shown, but window control buttons, icon on 
Unity panel and in window switcher would appear.

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https://bugs.launchpad.net/bugs/861143

Title:
  unity 3d firefox window borders disappear

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