Do you have this file?

/usr/share/glib-2.0/schemas/org.gtk.Settings.Debug.gschema.xml

If so then try:
sudo glib-compile-schemas /usr/share/glib-2.0/schemas/

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https://bugs.launchpad.net/bugs/1523929

Title:
  "No such schema 'org.gtk.Settings.Debug'" error upon trying to
  activate GTKInspector shortcuts

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