What is wrong with using DIAMOND OPERATOR?
"wrong" is strong wording and goes beyond what I suggested or implied, but it's not clear to a user of Unicode that it's the right fit either. There are a couple of indicators factoring in:

 * The charts mention modal logic in conjunction with ◻ (U+25FB) and ⟠
   (U+27E0) but not with ⋄ (U+22C4).
 * The glyph in the code charts is tiny (and that of Cambria Math is
   tiny as well). Typographically you see various things (a lozenge,
   fallback to letter-M) in esp older books, but it feels like it's
   meant to be an orthogonal diamond of perhaps slightly less area than
   the box but descending a little above and below the box, which is
   somewhat taller than x-height. The book by {Blackburn, de Rijke,
   Venema} has glyphs that look right. This is more than a guess: it
   makes sense if they have similar visual weight, as they are –
   literally – defined to be duals of one another; but whether you can
   make them geometrically congruent symbols of equal area I haven't
   tested (this might have the diamond ascend too far).
 * The vague notion of "operator" (a word with different meanings in
   math, from /logical relation/  to /[non-logical/non-relational]
   mapping of type A×A→A or perhaps A×A→B/  to /(linear) map (between
   say vector spaces) in linear algebra/) in this context (in the code
   charts) seems to refer to something like my middle meaning, which is
   likely to use a smaller symbol around x-height in placement and
   dimensions.
 * The glyph of ⬦ (U+2B26) seems to have a more appropriate name, but
   in the charts I like ◇ U+25C7. The differently sized square-like
   symbols are hard to semantically tell apart in/from the charts anyway.
 * These symbols are the first two visually distinct ones you define in
   modal logic, so they're well-known and standardized in meaning for
   anyone who had had contact with the field. It's surprising they're
   not explicitly named in the charts. (There's stuff like the outdated
   horseshoe for logical implication popping up in the relevant books,
   but that is a leftover or outdated logic notation in general.) So
   for box and diamond it's quite reasonable to be expecting a standard
   math font to provide them just right out of the box; for whatever
   commonly used box-like symbols in math there are, one would assume
   that there are corresponding codepoints; otherwise you'd have to
   choose a different font.


Stephan

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