Hi Mauro,

Environ has the possibility to define a confining potential (keyword 
env_confine, only available in Environ 1.1). Although this feature was added 
for other purposes, we found that it helps keeping solvent molecules on the 
surface of a slab, without adding too much of a constraint. As you know, 
Environ is not compatible with ESM, but it should allow similar simulations of 
charged surfaces in electrolyte media.

Best,

Oliviero Andreussi
Department of Physics
University of North Texas
www.materialab.org

On Jun 26, 2020, at 5:58 PM, Mauro Sgroi <[email protected]> wrote:


Dear all,
I'm trying to simulate the interface between a charged doped graphene layer and 
a liquid electrolyte.
I would like to treat the solvent explicitly. So I should place some molecules 
of the solvent in the vacuum region of my slab model.
I've seen that with the OpenMX code it is possible to use the ESM method and 
define a potential to confine the liquid in a certain portion of the space 
between periodic images of the substrate. This prevents the liquid filling all 
the vacuum space of the supercell during MD.

Here is an explicative figure:
http://www.openmx-square.org/openmx_man3.7/node118.html<https://nam04.safelinks.protection.outlook.com/?url=http%3A%2F%2Fwww.openmx-square.org%2Fopenmx_man3.7%2Fnode118.html&data=02%7C01%7Coliviero.andreussi%40unt.edu%7Ce629d94e0041405af89e08d81a246595%7C70de199207c6480fa318a1afcba03983%7C0%7C0%7C637288090952975915&sdata=rGmUkDZbaQXtQrzhOC4Y6qUf7dZYo1kaPjQ38B3q2HQ%3D&reserved=0>

Is something similar implemented in Quantum Espresso?
Or is it possible to obtain it using constraints on the coordinates?

Thanks a lot in advance and best regards,
Mauro Sgroi.
Centro Ricerche FIAT.


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