Dear community,

I am interested in calculating the CrBr3 J exchange parameters of an 
anisotropic Heisenberg Hamiltonian as it is shown in this paper: 
https://doi.org/10.1039/C2DT31662E (Equations A16 and A17 on section D in the 
appendix)
 My idea would be to perform a collinear spin-polarized scf calculation (i.e. 
using scalar relativistic pseudopotentials), and then perform a non collinear 
nscf calculation for each of the spin configurations, following a similar 
procedure as in the MAE example 
https://gitlab.com/QEF/q-e/-/tree/f184591e9f34cfcc7767505a23977a92286e8ba6/PP/examples/ForceTheorem_example
Would this be reasonable or should I do a non collinear scf calculation for 
each scenario and extract Jxx,Jyy,Jzz from the total energies? Has someone 
experience with this kind of calculations?

Thank you in advance
Dorye L. Esteras 
Predoctoral researcher
University of Valencia
 
 
 

 


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