Dear Thomas Brumme,

I'm not familiar with the +U method and this is a general view.

- One possibility is the difference in the relaxation route achieving
  the most stable state. In some cases, the system may be trapped in
  quasi stable state.

  Suppose that you get structure A in QE and structure B in VASP, both
  starting from the original structure G, you can compare the relative
  energies by performing the static scf calculations for A, B, and G.

  If both of the codes return the same order of energies, such as E(A)
  < E(B) < E(G), you can safely identify the stable structure (in this
  case the structure A). Be careful about the k-points and cutoff 
  energies. The number of PWs of A must be different from that
  of B and you must maintain the accuracy by increasing the k-points
  and the cutoff.

- Are you using dense k-points mesh and high cutoff energies in the
  relaxation process too?

- Of course the difference of the pseudo/PAW potentials may influence
  the results. This is the reason why the VASP has variety of
  pseudo/PAW potentials for some elements. Try the same calculations
  using different pseudo/PAW sets.

- Try the VASP relaxations without +U option. Will it return the same
  structure with +U?
  


> 2022/11/28 0:43、Thomas Brumme <[email protected]>のメール:

> In VASP the relaxation is not restricted and since both codes use more or 
> less the same theory, the difference might come from some
> details in the implementation of +U or from some things related to the 
> pseudo. Do you have any feeling/idea if changing to a different
> pseudo or something different concerning +U might influence the relaxation?
> 
> Kind regards
> 
> Thomas


西館数芽
Kazume NISHIDATE Ph.D

Department of Systems Innovation Engineering,
Graduate School of Science and Engineering, Iwate University
4-3-5 Ueda, Morioka, Iwate, 020-8551 JAPAN
Phone:+81-19-621-6391
[email protected], [email protected]
https://sites.google.com/site/nisidatelab/

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