At 13:09 16/09/2007, Rzepa, Henry wrote:

>With a given connection table, the initial refinement is much best done using
>mechanics, which will  NOT change the connection table.  PM3 could 
>well do this.
>
>We use the Ghemical system, but it currently implements only the  Tripos
>FF.  The UFF (universal force field) is a much better bet, but has not yet
>been implemented (the UFF IS documented, and open source).
>
>I realise none of this is off the shelf, but if
>
>Connection table => 3D  UFF coordinates  ==> PM6   ===>  Gaussian
>could be made to work, it would I think be the most efficient.
>
>(thinking about it,  the Gaussian program  DOES implement  UFF.
>
>so a Gaussian workflow of the type
>
>UFF
>
>--link1--
>
>PM3
>
>--link1--
>
>6-31G(d,p)    might be viable.   The --link1-- command by the way is how
>one daisy chains calculations together in Gaussian.

Excellent. In practice with PM5 we found that MOPAC rarely trashed 
organic structures and often refined them well. The main problems 
will be tetrahedral centres and cyclohexane rings (which often end up 
as twist-boats). I would filer these post hoc, shake them and recompute.

P.

>--
>
>Henry Rzepa.
>+44 (020) 7594 5774 (Voice); +44 (0870) 132 3747 (eFax); 
>[EMAIL PROTECTED] (iChat)
>  http://www.ch.ic.ac.uk/rzepa/ Dept. Chemistry, Imperial College 
> London, SW7  2AZ, UK.
>
>(Voracious anti-spam filter in operation for received email.
>If expected reply not received, please phone/fax).

Peter Murray-Rust
Unilever Centre for Molecular Sciences Informatics
University of Cambridge,
Lensfield Road,  Cambridge CB2 1EW, UK
+44-1223-763069 


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