http://onlinelibrary.wiley.com/doi/10.1002/grl.50441/abstract

Rap, A., C. E. Scott, D. V. Spracklen, N. Bellouin, P. M. Forster, K. S.
Carslaw, A. Schmidt, and G. Mann (2013), Natural aerosol direct and
indirect radiative effects, Geophys. Res. Lett., 40, 3297–3301,
doi:10.1002/grl.50441

Keywords:

radiative effect;natural aerosol

Abstract

Natural aerosol plays a significant role in the Earth's system due to its
ability to alter the radiative balance of the Earth. Here we use a global
aerosol microphysics model together with a radiative transfer model to
estimate radiative effects for five natural aerosol sources in the
present-day atmosphere: dimethyl sulfide (DMS), sea-salt, volcanoes,
monoterpenes, and wildfires. We calculate large annual global mean aerosol
direct and cloud albedo effects especially for DMS-derived sulfate (–0.23
Wm–2 and –0.76 Wm–2, respectively), volcanic sulfate (–0.21 Wm–2 and –0.61
Wm–2) and sea-salt (–0.44 Wm–2 and –0.04 Wm–2). The cloud albedo effect
responds nonlinearly to changes in emission source strengths. The natural
sources have both markedly different radiative efficiencies and
indirect/direct radiative effect ratios. Aerosol sources that contribute a
large number of small particles (DMS-derived and volcanic sulfate) are
highly effective at influencing cloud albedo per unit of aerosol mass
burden.

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