Poster's note: I've been asked to serialise the previously unposted
Phil Trans special issue papers, so here goes.  Anyone who gets sick
of this, please reply with "Shut up Andrew" in the subject line.

http://rsta.royalsocietypublishing.org/content/372/2031.toc

Stratospheric controlled perturbation experiment: a small-scale
experiment to improve understanding of the risks of solar
geoengineering

John A. Dykema, David W. Keith, James G. Anderson, Debra Weisenstein
DOI: 10.1098/rsta.2014.0059
Published 17 November 2014

Abstract

Although solar radiation management (SRM) through stratospheric
aerosol methods has the potential to mitigate impacts of climate
change, our current knowledge of stratospheric processes suggests that
these methods may entail significant risks. In addition to the risks
associated with current knowledge, the possibility of ‘unknown
unknowns’ exists that could significantly alter the risk assessment
relative to our current understanding. While laboratory
experimentation can improve the current state of knowledge and
atmospheric models can assess large-scale climate response, they
cannot capture possible unknown chemistry or represent the full range
of interactive atmospheric chemical physics. Small-scale, in situ
experimentation under well-regulated circumstances can begin to remove
some of these uncertainties. This experiment—provisionally titled the
stratospheric controlled perturbation experiment—is under development
and will only proceed with transparent and predominantly governmental
funding and independent risk assessment. We describe the scientific
and technical foundation for performing, under external oversight,
small-scale experiments to quantify the risks posed by SRM to
activation of halogen species and subsequent erosion of stratospheric
ozone. The paper's scope includes selection of the measurement
platform, relevant aspects of stratospheric meteorology, operational
considerations and instrument design and engineering.

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