Poster's note: if anyone has a quick visual summary of the discussed
techniques (e.g. a video), please post as a reply, or send to me for
reposting. A verbal summary is available in Appendix A of the paper.

http://rsta.royalsocietypublishing.org/content/372/2031/20140056

Factors determining the most efficient spray distribution for marine
cloud brightening

P. J. Connolly, G. B. McFiggans, R. Wood, A. Tsiamis
DOI: 10.1098/rsta.2014.0056
Published 17 November 2014

Abstract

We investigate the sensitivity of marine cloud brightening to the
properties of the added salt particle distribution using a cloud
parcel model, with an aim to address the question of, ‘what is the
most efficient particle size distribution that will produce a desired
cooling effect?’ We examine the effect that altering the aerosol
particle size distribution has on the activation and growth of drops,
i.e. the Twomey effect alone, and do not consider macrophysical cloud
responses that may enhance or mitigate the Twomey effect. For all four
spray generation methods considered, Rayleigh jet; Taylor cone jet;
supercritical fluid; and effervescent spray, salt particles within the
median dry diameter range Dm=30–100 nm are the most effective range of
sizes. The Rayleigh jet method is also the most energy efficient
overall. We also find that care needs to be taken when using droplet
activation parametrizations: for the concentrations considered, Aitken
particles do not result in a decrease in the total albedo, as was
found in a recent study, and such findings are likely to be a result
of the parametrizations' inability to simulate the effect of swollen
aerosol particles. Our findings suggest that interstitial aerosol
particles play a role in controlling the albedo rather than just the
activated cloud drops, which is an effect that the parametrization
methods do not consider.

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