http://onlinelibrary.wiley.com/doi/10.1002/2017JD026888/abstract

Sensitivity of aerosol distribution and climate response to stratospheric SO
2 injection locations†
<http://onlinelibrary.wiley.com/doi/10.1002/2017JD026888/abstract#jgrd54158-note-0001>
Authors

   - Simone Tilmes,
   - <[email protected]>
      - <http://orcid.org/0000-0002-6557-3569>
   1.
      2.
   -

      <[email protected]>

   
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   - Jadwiga H. Richter,
   - <http://orcid.org/0000-0001-7048-0781>
   1.

   
<http://onlinelibrary.wiley.com/advanced/search/results?searchRowCriteria%5B0%5D.fieldName=author&start=1&resultsPerPage=20&searchRowCriteria%5B0%5D.queryString=%22Jadwiga%20H.%20Richter%22>
   - Michael J. Mills,
   - <http://orcid.org/0000-0002-8054-1346>
   1.

   
<http://onlinelibrary.wiley.com/advanced/search/results?searchRowCriteria%5B0%5D.fieldName=author&start=1&resultsPerPage=20&searchRowCriteria%5B0%5D.queryString=%22Michael%20J.%20Mills%22>
   - Ben Kravitz,
   - <http://orcid.org/0000-0001-6318-1150>
   1.

   
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   - Douglas G. MacMartin,
   - <http://orcid.org/0000-0003-1987-9417>
   1.
      2.

   
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   - Francis Vitt,
   - <http://orcid.org/0000-0002-8684-214X>
   1.

   
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   - Joseph J. Tribbia,
   - <http://orcid.org/0000-0003-1639-9688>
   1.

   
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   - Jean-Francois Lamarque
   - <http://orcid.org/0000-0002-4225-5074>
   1.

   
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   - Accepted manuscript online:6 November 2017Full publication history
   
<http://onlinelibrary.wiley.com/doi/10.1002/2017JD026888/abstract#publication-history>
   - DOI:10.1002/2017JD026888  View/save citation
   
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   - †This article has been accepted for publication and undergone full
   peer review but has not been through the copyediting, typesetting,
   pagination and proofreading process, which may lead to differences between
   this version and the Version of Record. Please cite this article as doi:
   10.1002/2017jd026888

Abstract

Injection of SO2 into the stratosphere has been proposed as a method to in
part counteract anthropogenic climate change. So far, most studies
investigated injections at the equator or in a region in the tropics. Here,
we use CESM1(WACCM) to explore the impact of continuous single grid point SO
2injections at 7 different latitudes and 2 altitudes in the stratosphere on
aerosol distribution and climate. For each of the 14 locations, 3 different
constant SO2 emission rates were tested to identify linearity in aerosol
burden, aerosol optical depth, and climate effects. We found that
injections at 15° N and 15° S and at 25 km altitude have equal or greater
effect on radiation and surface temperature than injections at the equator.
Non-equatorial injections transport SO2 and sulfate aerosols more
efficiently into middle and high latitudes and result in particles of
smaller effective radius and larger aerosol burden in middle and high
latitudes. Injections at 15° S produce the largest increase in global
average aerosol optical depth, and increase the change in radiative forcing
per Tg SO2/yr by about 15% compared to equatorial injections. High altitude
injections at 15° N produce the largest reduction in global average
temperature of 0.2 degrees per Tg S/yr for the last 7 years of a ten year
experiment. Injections at higher altitude are generally more efficient at
reducing surface temperature, with the exception of large equatorial
injections of at least 12 Tg SO2/yr. These findings have important
implications for designing a strategy to counteract global climate change

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