Dear Tamas,

there are typically 3 effects that govern RF by stratospheric aerosols as a function of latitude for a given aerosol burden. Let's think in terms of solar zenith angle (one has then to integrate over SZA which is a function of latitude and season)

1/ insolation decreases with SZA as cos(theta) where theta is the SZA

2/ air mass increases with  SZA as 1/cos(theta), of course the effect this has breaks down at some point because of multiple scattering

3/ upscattering function also increases with SZA (because more forward scattering contributes to upscattering).

You could assume 1/ and 2/ cancel each other at first approximation, so because of 3/ there is indeed more RF at larger SZA. In fact there is an optimum around SZA=60° but that depends on the AOD and how much multiple scattering there is.

Now life is a bit more complicated, as transport and aerosol size varies also.

In any case, the climate response is not a copy-paste of the spatial distribution of the RF. It matters but not too much. And it matters more for rapid adjustments than for feedbacks. See eg https://agupubs.onlinelibrary.wiley.com/doi/full/10.1002/2013JD021110

Regards,

Olivier


Dear All,

I would like to ask for some useful references about sulfate aerosol geoengineering. 
Assuming some uniform aerosol coverage around the globe, at some height, with a certain 
vertical layer thickness, i would imagine that at higher latitudes the radiative forcing 
exerted by the aerosols is larger due to the longer distance of travel of sun rays 
through the aerosol "cloud". As a consequence, the latitude-dependence of the 
downward-directed radiative forcing should have an even larger gradient than solar 
irradiance. Therefore, I’m wondering how big mistake it is to model such a geoengineering 
scenario by dimming the sun.

Any feedback or reference would be much appreciated.

Thank you,

Tamas

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