*Poster's note: Old, but new to the list*

https://www.nature.com/articles/s41598-019-53595-3

*Authors*
Daniel J. Cziczo, Martin J. Wolf, Blaž Gasparini, Steffen Münch & Ulrike
Lohmann

*11 December 2019*

*Citation*: Cziczo, D.J., Wolf, M.J., Gasparini, B. *et al.* Unanticipated
Side Effects of Stratospheric Albedo Modification Proposals Due to Aerosol
Composition and Phase. *Sci Rep* 9, 18825 (2019).
https://doi.org/10.1038/s41598-019-53595-3
*Abstract*
The Earth has now warmed ~1.0 °C since the period 1850–1900, due in large
part to the anthropogenic addition of greenhouse gases to the atmosphere.
Most strategies to address this warming have called for a reduction of
emissions and, often, accompanying removal of greenhouse gases. Other
proposals suggest masking the increased radiative forcing by an increase in
particles and/or clouds to increase scattering of incoming solar radiation.
Two related recent proposals have suggested addition of calcite particles
to the stratosphere, which one model suggests may enhance ozone. Here we
show that the interaction of calcite with acidic materials in the
stratosphere results in a more complex aerosol than has been previously
considered, including aqueous and hydrate phases that can lead to ozone
loss. Our study suggests particle addition to the stratosphere could also
perturb global radiative balance by affecting high altitude cloud formation
and properties. Experimental and modeling results suggest particles will
act as the nucleation sites for polar stratospheric cloud ice and, after
sedimentation into the troposphere, impact cirrus clouds in the absence of
other efficient ice nucleating particles. These results show that an overly
simplistic set of assumptions regarding intentional particle emissions to
the atmosphere can lead to incorrect estimates of the radiative effect and
fail to identify unintended consequences.

*Source: nature*

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