https://www.nature.com/articles/s41612-024-00664-8

*Authors*
Hongwei Sun, Stephen Bourguet, Lan Luan & David Keith

*30 May 2024*

*Citations*: Sun, H., Bourguet, S., Luan, L. et al. Stratospheric transport
and tropospheric sink of solar geoengineering aerosol: a Lagrangian
analysis. npj Clim Atmos Sci 7, 115 (2024).
https://doi.org/10.1038/s41612-024-00664-8

*Abstract*
Stratospheric aerosol injection (SAI) aims to reflect solar radiation by
increasing the stratospheric aerosol burden. To understand how the
background circulation influences stratospheric transport of injected
particles, we use a Lagrangian trajectory model (lacking numerical
diffusion) to quantify particles’ number, flux, lifetime, and tropospheric
sinks from a SAI injection strategy under present-day conditions. While
particles are being injected, stratospheric particle number increases until
reaching a steady-state. During the steady-state, the time series of
particle number shows a dominant period of ~2 years (rather than a 1-year
cycle), suggesting modulation by the quasi-biannual oscillation. More than
half of particles, injected in the tropical lower stratosphere (15° S to
15° N, 65 hPa), undergo quasi-horizontal transport to the midlatitude. We
find a zonal asymmetry of particles’ tropospheric sinks that are co-located
with tropopause folding beneath the midlatitude jet stream, which can help
predict tropospheric impacts of SAI (e.g., cirrus cloud thinning).

[image: figure 1]
<https://www.nature.com/articles/s41612-024-00664-8/figures/1>

Time series of the number of particles (black line) in the stratosphere,
with three stages divided by the red dashed lines.
Evaluations of particle distribution and transport in the stratosphere.
[image: figure 4]
<https://www.nature.com/articles/s41612-024-00664-8/figures/4>

a Spatial distribution (latitude vs. altitude) of zonally integrated
particle number concentration (with a unit of particles per square
meter). b Particle
number N (red values with the unit of particles), number flux *F* (blue
values with a unit of particles per year), and lifetime *L* (purple values
with a unit of years) in or between different regions (black boxes) during
the steady-state stage (2005.01–2010.01). The injection rate is scaled to
100 particles per year and all other values are scaled correspondingly.
*Source: Nature*

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