https://egusphere.copernicus.org/preprints/2024/egusphere-2024-1111/

*Authors*
Robert G. Ryan, Lilani Toms-Hardman, Alexander Smirnov, Daniel Harrison,
and Robyn Schofield

*How to cite. *Ryan, R. G., Toms-Hardman, L., Smirnov, A., Harrison, D.,
and Schofield, R.: Measurement report: Aerosol vertical profiling over the
Southern Great Barrier Reef using lidar and MAX-DOAS measurements,
EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-1111, 2024.

*Received: 12 Apr 2024 – Discussion started: 28 Jun 2024*

*Abstract*
Aerosol vertical profile measurements were made using multi-axis
differential optical absorption spectroscopy (MAX-DOAS) and mini-Micropulse
LiDAR (MPL) at One Tree Island in the Southern Great Barrier Reef from
February to April 2023. This is an understudied location in terms of
atmospheric aerosols and chemistry but is growing in importance as multiple
research streams examine the influence of aerosols on radiation over the
Great Barrier Reef. Solar radiation management proposals require
regional-scale aerosol modelling, which is evaluated against aerosol
extinction and optical depth measurements, necessitating a thorough
understanding of measurements of these quantities. MPL aerosol retrieval
showed extinction-to-backscatter ratios (0.031 on average) and
depolarization ratios (0.015 on average) consistent with clean, unpolluted
Southern hemispheric marine aerosol. The maximum depolarization ratio
tended to be above the layer of maximum MPL backscatter, which is
attributed to dried sea-salt layers above the boundary layer. MAX-DOAS and
MPL extinction profiles show aerosol layers extending beyond 2 km altitude
in the middle of the day, but predominantly below 1 km at other times. We
also compared aerosol optical depth measurements from integrating the
MAX-DOAS and MPL extinction profiles, with observations from a hand-held
Microtops sun photometer. Mean aerosol optical depth (AOD) values across
the campaign compare well, being 0.083 ± 0.002 for the Microtops, 0.090 ±
0.032 for the MAX-DOAS and 0.104 ± 0.028 for the MPL. However, AOD
observations at a given time, and the AOD diurnal cycle, often varied
between instruments. This likely indicates strong horizontal inhomogeneity
in aerosol in this environment, a factor which makes it challenging to
accurately compare AOD estimates from different viewing geometries, but
which is important for future aerosol modelling studies in this region to
consider.

*Source: EGU Sphere*

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